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Atomic-Level Mechanisms Of Fast Relaxation In Metallic Glasses, Leo W. Zella Dec 2023

Atomic-Level Mechanisms Of Fast Relaxation In Metallic Glasses, Leo W. Zella

Doctoral Dissertations

Glasses are ubiquitous in daily life and have unique properties which are a consequence of the underlying disordered structure. By understanding the fundamental processes that govern these properties, we can modify glasses for desired applications. Key to understanding the structure-dynamics relationship in glasses is the variety of relaxation processes that exist below the glass transition temperature. Though these relaxations are well characterized with macroscopic experimental techniques, the microscopic nature of these relaxations is difficult to elucidate with experimental tools due to the requirements of timescale and spatial resolution. There remain many questions regarding the microscopic nature of relaxation in glass …


A Measurement Of Neutron Polarization And Transmission For The Nedm@Sns Experiment, Kavish Imam Dec 2023

A Measurement Of Neutron Polarization And Transmission For The Nedm@Sns Experiment, Kavish Imam

Doctoral Dissertations

The D.O.E Nuclear Science Advisory Committee Long Range Plan has called for experimental programs to explore fundamental symmetry violations and their implications in nuclear, particle and cosmological physics. The neutron electric dipole moment experiment at the Spallation Neutron Source (nEDM@SNS) aims to search for new physics in the Time-reversal (T) and Charge-Parity (CP) symmetry violating sector by setting a new limit on the nEDM down to a few x 10-28 e·cm using a novel cryogenic technique, which combines the unique properties of polarized Ultracold Neutrons (UCN), polarized 3He, and superfluid 4He. The experiment will employ a cryogenic …


Generative Adversarial Game With Tailored Quantum Feature Maps For Enhanced Classification, Anais Sandra Nguemto Guiawa Dec 2023

Generative Adversarial Game With Tailored Quantum Feature Maps For Enhanced Classification, Anais Sandra Nguemto Guiawa

Doctoral Dissertations

In the burgeoning field of quantum machine learning, the fusion of quantum computing and machine learning methodologies has sparked immense interest, particularly with the emergence of noisy intermediate-scale quantum (NISQ) devices. These devices hold the promise of achieving quantum advantage, but they grapple with limitations like constrained qubit counts, limited connectivity, operational noise, and a restricted set of operations. These challenges necessitate a strategic and deliberate approach to crafting effective quantum machine learning algorithms.

This dissertation revolves around an exploration of these challenges, presenting innovative strategies that tailor quantum algorithms and processes to seamlessly integrate with commercial quantum platforms. A …


Short Range Correlation Measurements In The Quasielastic Region With An 11 Gev Beam, Casey Morean Dec 2023

Short Range Correlation Measurements In The Quasielastic Region With An 11 Gev Beam, Casey Morean

Doctoral Dissertations

Electron scattering is a significant means of studying internal high momentum
nucleon and quark distributions in nuclei. Thomas Jefferson National Accelerator
Facility (JLab) with its 11GeV beam is capable of studying high momentum nucleons
with unmatched precision. The role of short range nucleon configurations and
quark distributions is significant for understanding the dynamics of nuclei and their
underlying components. Scattering cross section measurements in the kinematic
regime x > 1, where the free nucleon is forbidden, are sensitive to high momentum
nucleons, which are believed to come from short range correlations (SRCs). SRCs are
strongly interacting, high momentum nucleons with a …


Dinitrogen Functionalization Using A Molybdenum Atom: Bridging The Gap Between Small And Coordination Complexes Via Quantum Mechanical Methods, Maria Virginia White Aug 2023

Dinitrogen Functionalization Using A Molybdenum Atom: Bridging The Gap Between Small And Coordination Complexes Via Quantum Mechanical Methods, Maria Virginia White

Doctoral Dissertations

Chemistry devotes a significant amount of its research to understanding small molecule activation from an electronic structure perspective to help with the investigation of the reaction pathways of catalytically active substances that can promote biomimetic catalysis. A large portion of the energy used annually in our planet is used for the artificial nitrogen fixation (Haber-Bosch process), which renders dinitrogen activation a subject of study. Molybdenum, a fourth row transitional metal, has demonstrated its effectiveness as an essential component of the dinitrogen reduction catalytic process. To better understand the multiple dinitrogen molybdenum binding modes, the work described herein combines wave function …


Chirality, Symmetry-Breaking, And Chemical Substitution In Multiferroics, Kiman Park Aug 2023

Chirality, Symmetry-Breaking, And Chemical Substitution In Multiferroics, Kiman Park

Doctoral Dissertations

Multiferroic materials attract significant attention due to their potential utility in a broad range of device applications. The inclusion of heavy metal centers in these materials enhances their magnetoelectric properties, yielding fascinating physical phenomena such as the Dzyaloshinskii–Moriya interaction, nonreciprocal directional dichroism, enhancement of spin-phonon coupling, and spin-orbit-entangled ground states. This dissertation provides a comprehensive survey of magnetoelectric multiferroics containing heavy metal centers and explores spectroscopic techniques under extreme conditions. A microscopic examination of phase transitions, symmetry-breaking, and structure-property relationships enhances the fundamental understanding of coupling mechanisms.

In A2Mo3O8 (A = Fe, Zn, Ni, and Mn), we use optical spectroscopy …


Exploring Skyrmions Dynamics And Structure Using Neutron Scattering, W-L-Namila Chandula Liyanage Aug 2023

Exploring Skyrmions Dynamics And Structure Using Neutron Scattering, W-L-Namila Chandula Liyanage

Doctoral Dissertations

Magnetic skyrmions are topologically protected chiral spin textures with great potential for next-generation consumer technologies. These magnetic structures can be described as spins continuously wrapping into a closed coplanar loop, featuring a core and fencing perimeter with opposite out-of-plane orientations. While conventional depictions of magnetic skyrmions use a two-dimensional projection, recent research underscores the importance of their three-dimensional structure in determining their topology and stability. Magnetic skyrmions typically emerge just below the curie temperature of a magnetic material, creating what is known as a skyrmion pocket. In most materials the stability pocket is at low temperatures and finite fields, however …


Sub-Chandrasekhar Type Ia Supernovae Scenarios With Increased Pathways For Neutronization, Fernando Hernan Rivas May 2023

Sub-Chandrasekhar Type Ia Supernovae Scenarios With Increased Pathways For Neutronization, Fernando Hernan Rivas

Doctoral Dissertations

Type Ia supernovae are thermonuclear explosions of white dwarfs (WD), electron-degenerate cores of old intermediate mass stars(under 8$M_{\odot}$). Reaching energies of $10^{51}$\si{\erg}, they outshine whole galaxies as they synthesize and distribute most of the iron group elements (IGE; V, Cr, Mn, Fe, Co, Ni) into the interstellar medium, thus being one of the main agents in cosmic chemical evolution. Also, given their notably homogeneous lightcurves, they form the last step in the cosmic distance ladder outdistancing Cepheid variables by orders of magnitude. Though calibration of said lightcurves is dependent on a high number of confirmed events, the limits of statistical …


Fabrication, Measurements, And Modeling Of Semiconductor Radiation Detectors For Imaging And Detector Response Functions, Corey David Ahl May 2023

Fabrication, Measurements, And Modeling Of Semiconductor Radiation Detectors For Imaging And Detector Response Functions, Corey David Ahl

Doctoral Dissertations

In the first part of this dissertation, we cover the development of a diamond semiconductor alpha-tagging sensor for associated particle imaging to solve challenges with currently employed scintillators. The alpha-tagging sensor is a double-sided strip detector made from polycrystalline CVD diamond. The performance goals of the alpha-tagging sensor are 700-picosecond timing resolution and 0.5 mm spatial resolution. A literature review summarizes the methodology, goals, and challenges in associated particle imaging. The history and current state of alpha-tagging sensors, followed by the properties of diamond semiconductors are discussed to close the literature review. The materials and methods used to calibrate the …


Path Integral Monte Carlo For Entanglement In Bosonic Lattices At T = 0, Emanuel Casiano-Diaz May 2023

Path Integral Monte Carlo For Entanglement In Bosonic Lattices At T = 0, Emanuel Casiano-Diaz

Doctoral Dissertations

Path-Integral Monte Carlo Worm Algorithm is one of many Quantum Monte Carlo (QMC) methods that serve as powerful tools for the simulation of quantum many-body systems. Developed in the late 90’s, this algorithm has been used with great success to study a wide array of physical models where exact calculation of observables is not possible due to the exponential size of the Hilbert space. One type of systems that have eluded PIMC-WA implementation are lattice models at zero temperature, which are of relevance in experimental settings, such as in optical lattices of ultra-cold atoms. In this thesis, we develop a …


Pointing Control And Stabilization Of The High-Energy Uv Laser For Laser-Assisted Charge Exchange, Martin Joseph Kay May 2023

Pointing Control And Stabilization Of The High-Energy Uv Laser For Laser-Assisted Charge Exchange, Martin Joseph Kay

Doctoral Dissertations

Laser-Assisted Charge Exchange (LACE) is an experimental method of charge exchange injection into a proton accumulator ring that is being developed at the Spallation Neutron Source (SNS) in Oak Ridge National Laboratory (ORNL) as an alternative to hazardous injection foils. The current scheme of LACE requires a high-energy, low-repetition-rate UV (355 nm) laser beam (140 mJ pulses at 10 Hz) to be transported over 65 meters to the laser-particle interaction point (IP) in a high-radiation area of the accelerator. Thermal effects and other disturbances along the free-space laser transport line cause the beam to slowly drift away from the IP …


Total Absorption Spectroscopy Of Mo-106 And Tc-106, Michael Cooper May 2023

Total Absorption Spectroscopy Of Mo-106 And Tc-106, Michael Cooper

Doctoral Dissertations

Total absorption spectroscopy is a method of gamma-ray spectroscopy that has gained prominence in the past several decades, as nuclear data revisions are performed on older nuclear data, which is often incomplete. A strong understanding of underlying nuclear data, particularly fission and beta decay data, is essential for nuclear reactors and nuclear fuel decay heat. This PhD work involves the analysis of fission fragments 106Mo [Mo-106] and 106Tc [Tc-106]. These neutron rich isotopes contribute upwards of 6% of the cumulative fission yield of 241Pu [Pu-241] fission, and 4% of 239Pu [Pu-239] fission. Prior data for these two fission fragments only …


Unlocking The Potential Of Machine Learning In The Derivation Of Low-Energy Models For Metallic Magnets, Vikram Sharma May 2023

Unlocking The Potential Of Machine Learning In The Derivation Of Low-Energy Models For Metallic Magnets, Vikram Sharma

Doctoral Dissertations

Condensed matter physics often grapples with complex many-particle problems lacking definitive closed-form solutions, necessitating approximation strategies to investigate low-energy sectors of the Hilbert space. Perturbation theory, though widely used for this purpose, is limited when expansion terms diverge. This work introduces a machine learning (ML) assisted protocol to extract effective low-energy models for lattice models of fermions interacting with classical fields, specifically focusing on the Kondo Lattice Model (KLM).

Skyrmions, featuring whirling spin texture and topological protection, are promising candidates for future spintronic devices. Materials featuring conduction electrons coupled to localized $f$-electrons' net moment are ideal for realizing skyrmions and …


Neutrino Physics At A Research Reactor: Backgrounds And Analysis, Blaine Alexander Heffron May 2023

Neutrino Physics At A Research Reactor: Backgrounds And Analysis, Blaine Alexander Heffron

Doctoral Dissertations

The field of neutrino physics has a rich history and is currently the subject of much active research. The discovery of neutrino oscillations led to the conclusion that neutrinos have mass which was in contradiction to the Standard Model. Now researchers are investigating a number of open questions regarding neutrino properties such as their mass values or the existence of CP violation in the weak interaction. In order to answer these questions experimental and analytical techniques of neutrino detection are becoming more advanced, entering into an era of precision neutrino detection.

Nuclear reactors as a source of antineutrinos have played …