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Zirconium Diboride, Hexagonal Boron Nitride, And Amorphous Alumina Thin Films For High Temperature Applications, David Murdock Stewart
Zirconium Diboride, Hexagonal Boron Nitride, And Amorphous Alumina Thin Films For High Temperature Applications, David Murdock Stewart
Electronic Theses and Dissertations
The use of microelectronic sensors and actuators in harsh, high temperature environments, such as power plants, turbine engines, and industrial manufacturing, could greatly improve the safety, reliability, and energy efficiency of these processes. The primary challenge in implementing this technology is the breakdown and degradation of thin films used in fabricating these devices when exposed to high temperatures >800 °C and oxidizing atmospheres. Zirconium diboride, hexagonal boron nitride, and amorphous alumina are candidate materials for use as thin film sensor components due to their high melting temperatures and stable phases. Zirconium diboride thin films have metallic-like electrical conductivity and remain …
Roles Of Siphon Flows In Suspension Feeding, Kevin Du Clos
Roles Of Siphon Flows In Suspension Feeding, Kevin Du Clos
Electronic Theses and Dissertations
Benthic marine suspension feeders provide an important link between benthic and pelagic ecosystems. The strength of this link is determined by suspension-feeding rates. Many studies have measured suspension-feeding rates using indirect clearance-rate methods, which are based on the depletion of suspended particles. Direct methods that measure the flow of water itself are less common, but they can be more broadly applied because clearance-rate measurements are affected by properties of the cleared particles. We present pumping rates for three species of suspension feeders, the clams Mya arenaria and Mercenaria mercenaria and the tunicate Ciona intestinalis, calculated using a direct method …
Microstructural Analysis Of Thermoelastic Response, Nonlinear Creep, And Pervasive Cracking In Heterogeneous Materials, Alden C. Cook
Microstructural Analysis Of Thermoelastic Response, Nonlinear Creep, And Pervasive Cracking In Heterogeneous Materials, Alden C. Cook
Electronic Theses and Dissertations
This dissertation is concerned with the development of robust numerical solution procedures for the generalized micromechanical analysis of linear and nonlinear constitutive behavior in heterogeneous materials. Although the methods developed are applicable in many engineering, geological, and materials science fields, three main areas are explored in this work. First, a numerical methodology is presented for the thermomechanical analysis of heterogeneous materials with a special focus on real polycrystalline microstructures obtained using electron backscatter diffraction techniques. Asymptotic expansion homogenization and finite element analysis are employed for micromechanical analysis of polycrystalline materials. Effective thermoelastic properties of polycrystalline materials are determined and compared …
Investigating High Speed Localization Microscopy Through Experimental Methods, Data Processing Methods, And Applications Of Localization Microscopy To Biological Questions, Andrew J. Nelson
Electronic Theses and Dissertations
Fluorescence Photoactivation Localization Microscopy(FPALM) and other super resolution localization microscopy techniques can resolve structures with nanoscale resolution. Unlike techniques of electron microscopy, they are also compatible with live cell and live animal studies, making FPALM and related techniques ideal for answering questions about the dynamic nature of molecular biology in living systems. Many processes in biology occur on rapid sub second time scales requiring the imaging technique to be capable of resolving these processes not just with a high enough spatial resolution, but with an appropriate temporal resolution. To that end, this Dissertation in part investigates high speed FPALM as …
A Study Of The Radiative Pion Capture Process As A Background To The Search For Muon To Electron Conversion With The Mu2e Experiment., Jacob Colston
A Study Of The Radiative Pion Capture Process As A Background To The Search For Muon To Electron Conversion With The Mu2e Experiment., Jacob Colston
Electronic Theses and Dissertations
This thesis will introduce radiative pion capture (RPC), a process which can produce a fake signal in a search for the coherent conversion of a muon to an electron in the presence of a nucleus. There will be a brief introduction to standard model (SM) physics, as well as some more in-depth discussion of the relevant high energy physics at the Mu2e experiment. We will discuss charged lepton flavor violation (CLFV), as well as Supersymmetry, which predicts CLFV at higher intensities than the SM prediction. A description of the RPC process follows, including the external and internal conversions in pion …
Materials Design And Band Gap Engineering Of Complex Nanostructures Using A Semi-Empirical Approach : Low Dimensional Boron Nanostructures, H-Bn Sheet With Graphene Domains And Holey Graphene., Cherno Baba Kah
Electronic Theses and Dissertations
This dissertation will explore the potential of a semi-empirical Hamiltonian, developed by the research group at the University of Louisville, in predicting the existence of new families of low-dimensional boron nanostructures based on icosahedral α-B12 clusters, and in tuning the band gaps of h-BN sheets with graphene domains and holey graphene. This semi-empirical Hamiltonian models electron-electron and electron-ion interactions using environment-dependent (ED) functions, and ion-ion interactions via usual pairwise terms. Additional features of our approach are that it uses a linear combination of atomic orbitals (LCAO) framework to describe the Hamiltonian and it calculates the charge distribution around a …
Strategies Of Balancing: Regulation Of Posture As A Complex Phenomenon, Allison Leich Hilbun
Strategies Of Balancing: Regulation Of Posture As A Complex Phenomenon, Allison Leich Hilbun
Electronic Theses and Dissertations
The complexity of the interface between the muscular system and the nervous system is still elusive. We investigated how the neuromuscular system functions and how it is influenced by various perturbations. Postural stability was selected as the model system, because this system provides complex output, which could indicate underlying mechanisms and feedback loops of the neuromuscular system. We hypothesized that aging, physical pain, and mental and physical perturbations affect balancing strategy, and based on these observations, we constructed a model that simulates many aspects of the neuromuscular system. Our results show that aging changes the control strategy of balancing from …
Synthesis, Characterization, And Electronic Properties Of Novel 2d Materials : Transition Metal Dichalcogenides And Phosphorene., George Anderson
Synthesis, Characterization, And Electronic Properties Of Novel 2d Materials : Transition Metal Dichalcogenides And Phosphorene., George Anderson
Electronic Theses and Dissertations
Scaling electronic devices has become paramount. The current work builds upon scaling efforts by developing novel synthesis methods and next generation sensing devices based on 2D materials. A new combination method utilizing thermal evaporation and chemical vapor deposition was developed and analyzed to show the possibilities of Transition Metal Dichalcogenide monolayers and heterostructures. The materials produced from the above process showed high degrees of compositional control in both spatial dimensions and chemical structure. Characterization shows controlled fabrication of heterostructures, which may pave the way for future band gap engineering possibilities. In addition, Phosphorene based field effect transistors, photodetectors, and gas …
Self-Assembly Of Rous Sarcoma Virus Capsid Protein, Probed By Solid-State Nmr And Tem, Jaekyun Jeon
Self-Assembly Of Rous Sarcoma Virus Capsid Protein, Probed By Solid-State Nmr And Tem, Jaekyun Jeon
Electronic Theses and Dissertations
The retroviral capsid protein (CA) is derived from the cleavage of Gag polyprotein during the maturation process, and self-assembles into a polymorphic fullerene-like shell encasing the viral genome materials. The orthoretroviral CAs, for instance, Human Immunodeficiency Virus (HIV) and Rous Sarcoma Virus (RSV) CA, has little similarity in their sequence composition but a common 3D structure. They form distinct capsid assembly in vivo and a range of similar assemblies in vitro. Due to the substantial polymorphism, such assemblies are not amenable for conventional structural biology techniques such as X-ray diffraction crystallography and cryo-electron microscopy (cryo-EM). Solid-state NMR spectroscopy is the …
Ultrafast Mechanisms Of Nonlinear Refraction And Two-Photon Photochromism, Peng Zhao
Ultrafast Mechanisms Of Nonlinear Refraction And Two-Photon Photochromism, Peng Zhao
Electronic Theses and Dissertations
Derived from a material's third-order nonlinearity, nonlinear refraction (NLR) occurs at any wavelength in any material, and may exhibit noninstantaneous dynamics depending on its physical origins. The main subject of this dissertation is to investigate the underlying mechanisms responsible for the NLR response in different phases of matter, e.g. liquids, gases, and semiconductors, by extensively using our recently developed ultrafast Beam Deflection (BD) technique. An additional subject includes the characterization of a novel two-photon photochromic molecule. In molecular liquids, the major nonlinear optical (NLO) response can be decomposed into a nearly instantaneous bound-electronic NLR (Kerr effect), originating from the real …
Hybrid Integrated Photonic Platforms And Devices, Jeffrey Chiles
Hybrid Integrated Photonic Platforms And Devices, Jeffrey Chiles
Electronic Theses and Dissertations
Integrated photonics has the potential to revolutionize optical systems by achieving drastic reductions in their size, weight and power. Remote spectroscopy, free-space communications and high-speed telecommunications are critical applications that would benefit directly from these advancements. However, many such applications require extremely wide spectral bandwidths, leading to significant challenges in their integration. The choice of integrated platform influences the optical transparency and functionality which can be ultimately achieved. In this work, several new platforms and technologies have been developed to meet these needs. First, the silicon-on-lithium-niobate (SiLN) platform is discussed, on which the first compact, integrated electro-optic modulator in the …
Electrical Parasitic Bandwidth Limitations Of Oxide-Free Lithographic Vertical-Cavity Surface-Emitting Lasers, Xu Yang
Electronic Theses and Dissertations
Nowadays, Vertical-Cavity Surface-Emitting Lasers (VCSELs) are the most popular optical sources in short-reach data communications. In the commercial oxide VCSEL technology, an oxide aperture is created inside resonant cavity in realizing good mode and current confinement, however, high electrical resistance comes along with forming the oxide aperture and the electrical parasitic bandwidth becomes the main limitation in modulation speed. In this report, electrical bandwidths of oxide-free lithographic VCSELs have been studied along with their general lasing properties. Due to the new ways of fabricating the aperture, record low resistances have been achieved in oxide-free lithographic VCSELs with various sizes, while …
Broad Bandwidth Optical Frequency Combs From Low Noise, High Repetition Rate Semiconductor Mode-Locked Lasers, Anthony Klee
Broad Bandwidth Optical Frequency Combs From Low Noise, High Repetition Rate Semiconductor Mode-Locked Lasers, Anthony Klee
Electronic Theses and Dissertations
Mode-locked lasers have numerous applications in the areas of communications, spectroscopy, and frequency metrology. Harmonically mode-locked semiconductor lasers with external ring cavities offer a unique combination of benefits in that they can produce high repetition rate pulse trains with low timing jitter, achieve narrow axial mode linewidths, have the potential for entire monolithic integration on-chip, feature high wall-plug efficiency due to direct electrical pumping, and can be engineered to operate in different wavelength bands of interest. However, lasers based on InP/InGaAsP quantum well devices which operate in the important telecom C-band have thus far been relatively limited in bandwidth as …
Dynamical Formation Of Protoplanetesimals, Akbar Whizin
Dynamical Formation Of Protoplanetesimals, Akbar Whizin
Electronic Theses and Dissertations
The seeds of planetesimals that formed in the gaseous protoplanetary disk (PPD) have many barriers to overcome in their growth from millimeter to meter-sized and larger bodies. Centimeter-sized aggregates are weakly bound and self-gravity is almost non-existent so surface forces play a critical role in holding small loosely-bound rubble-piles together. Their orbital motions and effects form disk processes impart relative velocities leading to collisions so understanding the macroscopic disk environment is also necessary. To this end we analyze the dynamics of particles in Saturn's F ring as an analogue to understanding the orbital evolution of proto-planetesimals embedded in a PPD. …
Investigating The Predictive Power Of Student Characteristics On Success In Studio-Mode, Algebra-Based Introductory Physics Courses, Jarrad Pond
Electronic Theses and Dissertations
As part of a project to explore the differential success of similar implementations of the studio-mode of physics instruction, the objective of this work is to investigate the characteristics of students enrolled in algebra-based, studio-mode introductory physics courses at various universities in order to evaluate what effects these characteristics have on different measures of student success, such as gains in conceptual knowledge, shifts to more favorable attitudes toward physics, and final course grades. In my analysis, I explore the strategic self-regulatory, motivational, and demographic characteristics of students in algebra-based, studio-mode physics courses at three universities: the University of Central Florida …
Design And Engineering Of Ultrafast Amplifier Systems, Benjamin Webb
Design And Engineering Of Ultrafast Amplifier Systems, Benjamin Webb
Electronic Theses and Dissertations
Recently, the design and engineering of ultrafast laser systems have led to an extraordinary increase in laser power and performance which have brought about advances in many fields such as medicine, material processing, communications, remote sensing, spectroscopy, nonlinear optics, and atomic physics. In this work, several ultrafast amplification techniques -- including chirped-pulse amplification (CPA), optical parametric chirped-pulse amplification (OPCPA), and divided-pulse amplification (DPA) -- are described and demonstrated in the design and construction of two ultrafast laser facilities. An existing Ti:Sapphire laser system was completely redesigned with an increased power of 10 TW for experiments capable of generating hundreds of …
Optical Parity Time Metasurface Structures, Ahmed El Halawany
Optical Parity Time Metasurface Structures, Ahmed El Halawany
Electronic Theses and Dissertations
In the last few years, optics has witnessed the emergence of two fields namely metasurfaces and parity-time (PT) symmetry. Optical metasurfaces are engineered structures that provide unique responses to electromagnetic waves, absent in natural materials. Optical metasurfaces are known for their reduced dimensionality i.e. subwavelength and consequently lower losses are anticipated. The other paradigm is the PT symmetric materials, also known as photonic synthetic matter. PT symmetry has emerged from quantum mechanics when a new class of non-Hermitian Hamiltonian quantum systems was highlighted to have real eigenvalues, hence eradicating Hermiticity of the Hamiltonian as an essential condition to the existence …
Internal Degrees Of Freedom And Spin Transitions In Single Molecule Magnets, James Atkinson
Internal Degrees Of Freedom And Spin Transitions In Single Molecule Magnets, James Atkinson
Electronic Theses and Dissertations
This thesis covers a range of work detailing the transitions between spin eigenstates in molecular magnet systems. Broadly speaking, these transitions can be divided into two kinds: Those that involve a the tunneling of spin through a potential barrier to a resonant state on the other side, a phenomenon known as quantum tunneling of magnetization, and those that occur through the absorption or emission of a photon. In this latter case, the energy of the photon must match the difference between two eigenstates with a difference in angular momentum of ?. We will detail research performed on single molecule magnets, …
Monolithically Integrated Inp-Based Unidirectional Circulators Utilizing Non-Hermiticity And Nonlinearity, Parinaz Aleahmad
Monolithically Integrated Inp-Based Unidirectional Circulators Utilizing Non-Hermiticity And Nonlinearity, Parinaz Aleahmad
Electronic Theses and Dissertations
The need to integrate critical optical components on a single chip has been an ongoing quest in both optoelectronics and optical communication systems. Among the possible devices, elements supporting non-reciprocal transmission are of great interest for applications where signal routing and isolation is required. In this respect, breaking reciprocity is typically accomplished via Faraday rotation through appropriate magneto-optical arrangements. Unfortunately, standard light emitting optoelectronic materials like for example III-V semiconductors, lack magneto-optical properties and hence cannot be directly used in this capacity. To address these issues, a number of different tactics have been attempted in the last few years. These …
Coupling Of Laser Beams For Filament Propagation, Daniel Kepler
Coupling Of Laser Beams For Filament Propagation, Daniel Kepler
Electronic Theses and Dissertations
Laser filamentation is a nonlinear process involving high-energy, ultrashort pulses that create narrow, non-diffracting structures over many times the Raleigh length. While many of the characteristics of filaments can vary greatly depending on the physical parameters used to create them, they share several defining features: a high intensity core, a lower intensity cladding of photons that serves as an energy reservoir to the core, and spectral broadening into a supercontinuum. While there have been many studies on the creation and control of multiple filaments from one laser pulse and a few studies on the interaction of two single filaments, many …
Model Nanocatalysts With Tunable Reactivity: Tailoring The Structure And Surface Chemistry Of Nanomaterials For Energy And Alternative Fuels Catalysis, Hemma Mistry
Electronic Theses and Dissertations
One of the most pressing challenges of our time is meeting growing global energy demands while limiting human impact on the environment. To meet this challenge, new catalysts are needed to enable carbon neutral energy production processes and low cost synthesis of alternative fuels. In order to design new catalysts for such processes, fundamental understanding is needed on how the structural and chemical properties of nanostructured materials influences their surface chemistry. In this dissertation, I explore how the properties of nanoparticles, such as particle size, shape, composition, and chemical state, can be used to tune their reactivity. For this work, …
Multi-Purpose Device For Analyzing And Measuring Ultra-Short Pulses, Naman Anilkumar Mehta
Multi-Purpose Device For Analyzing And Measuring Ultra-Short Pulses, Naman Anilkumar Mehta
Electronic Theses and Dissertations
Intensity auto correlator is device to measure pulse widths of ultrashort pulses on the order of picoseconds and femtoseconds. I have built an in-house, compact, portable, industry standard intensity auto correlator for measuring ultrashort pulse-widths. My device is suitable for pulse-widths from 500 ps to 50 fs. The impetus for developing this instrument stemmed from our development of a multicore-fiber laser for high power laser applications, which also produces very short pulses that cannot be measured with an oscilloscope. As techniques for measuring short pulse-widths have been well studied, what made my journey exciting was the process of taking an …
Size, Shape, Composition And Chemical State Effects In Nanocatalysis, Mahdi Ahmadi
Size, Shape, Composition And Chemical State Effects In Nanocatalysis, Mahdi Ahmadi
Electronic Theses and Dissertations
The field of nanocatalysis has gained significant attention in the last decades due to the numerous industrial applications of nanosized catalysts. Size, shape, structure, and composition of the nanoparticles (NPs) are the parameters that can affect the reactivity, selectivity and stability of nanocatalysts. Therefore, understanding how these parameters affect the catalytic properties of these systems is required in order to engineer them with a given desired performance. It is also important to gain insight into the structural evolution of the NP catalysts under different reaction conditions to design catalysts with long durability under reaction condition. In this dissertation a synergistic …
Conformations And Dynamics Of Semi-Flexible Polymers, Aiqun Huang
Conformations And Dynamics Of Semi-Flexible Polymers, Aiqun Huang
Electronic Theses and Dissertations
In this dissertation, we investigate the conformations, transverse fluctuations and dynamics of two-dimensional (2D) semi-flexible polymers both in the bulk and under channel confinement. We present unified scaling relations in regard to various quantities of interest for a broad range of combinations of chain length and chain stiffness using Langevin dynamics simulation. We also present a three-dimensional (3D) heterogeneous semi-flexible chain model for a double stranded DNA (dsDNA). Our model not only confirms the established findings for homogeneous dsDNA, but also predicts new physical phenomenon for heterogeneous dsDNA. The problems studied in this dissertation are relevant to analysis of the …
Saturn's Rings: Measuring Particle Size Distributions Using Cassini Uvis Occultation Data, Tracy Becker
Saturn's Rings: Measuring Particle Size Distributions Using Cassini Uvis Occultation Data, Tracy Becker
Electronic Theses and Dissertations
Since its arrival to Saturn in 2004, the Cassini spacecraft has utilized its suite of sophisticated instruments to further our understanding of the Saturnian ring system. We analyze occultation data from Cassini's Ultraviolet Imaging Spectrograph (UVIS) in order to measure the particle size distribution and place limits on the minimum particle sizes in Saturn's rings. Throughout the ring system, particle accretion is countered by collisional and tidal disruption and Keplerian shear. Therefore, the particle size distribution of the rings is continually evolving. The presence of sub-centimeter particles, which have short lifetimes due to these processes, is indicative of ongoing dynamics …
Impact Of Gamma-Irradiation On The Characteristics Of Iii-N/Gan Based High Electron Mobility Transistors, Anupama Yadav
Impact Of Gamma-Irradiation On The Characteristics Of Iii-N/Gan Based High Electron Mobility Transistors, Anupama Yadav
Electronic Theses and Dissertations
In this study, the fundamental properties of AlGaN/GaN based High Electron Mobility Transistors (HEMTs) have been investigated in order to optimize their performance in radiation harsh environment. AlGaN/GaN HEMTs were irradiated with 60Co gamma-rays to doses up to 1000 Gy, and the effects of irradiation on the devices' transport and optical properties were analyzed. Understanding the radiation affects in HEMTs devices, on carrier transport, recombination rates and traps creation play a significant role in development and design of radiation resistant semiconductor components for different applications. Electrical testing combined with temperature dependent Electron Beam Induced Current (EBIC) that we used in …
Molecular Mechanisms Of Protein Thermal Stability, Lucas Sawle
Molecular Mechanisms Of Protein Thermal Stability, Lucas Sawle
Electronic Theses and Dissertations
Organisms that thrive under extreme conditions, such as high salt concentration, low pH, or high temperature, provide an opportunity to investigate the molecular and cellular strategies these organisms have adapted to survive in their harsh environments. Thermophilic proteins, those extracted from organisms that live at high temperature, maintain their structure and function at much higher temperatures compared to their mesophilic counterparts, found in organisms that live near room temperature. Thermophilic and mesophilic homolog protein pairs have identical functionality, and show a high degree of structural and sequential similarity, but differ significantly in their response to high temperature. Addressing the principles …
Thermal Effects On Spin Currents In Non-Local Metallic Spin Valves, Alex Hojem
Thermal Effects On Spin Currents In Non-Local Metallic Spin Valves, Alex Hojem
Electronic Theses and Dissertations
The study of non-local spin valves (NLSVs) has recently proven to be a fertile area for both applied and fundamental research in nanomagnetism due to the unique ability to separate charge currents and spin currents. NLSVs may also prove essential for a new class of high-density hard disk read heads due to their favorable scalability. Recent studies have shown thermal effects created by high current densities play a significant role in the response of NLSVs. These thermal effects also provide the opportunity to create a pure spin current from thermal gradients via a mechanism call the spin dependent Seebeck effect …
Temperature And Pressure Effects On Elastic Properties Of Relaxor Ferroelectrics And Thermoelectrics: A Resonant Ultrasound Spectroscopy Study, Sumudu Tennakoon
Temperature And Pressure Effects On Elastic Properties Of Relaxor Ferroelectrics And Thermoelectrics: A Resonant Ultrasound Spectroscopy Study, Sumudu Tennakoon
Electronic Theses and Dissertations
Relaxor ferroelectric lead magnesium niobate-lead titanate (PMN-PT) material exhibits exceptional electromechanical properties. The material undergoes a series of structural phase transitions with changes in temperature and the chemical composition. The work covered in this dissertation seek to gain insight into the phase diagram of PMN-PT using temperature and pressure dependence of the elastic properties. Single crystal PMN-PT with a composition near morphotropic phase boundary (MPB) was investigated using a resonant ultrasound spectroscopy (RUS) methodologies in the temperature range of 293 K - 800 K and the pressure range from near vacuum to 3.4 MPa. At atmospheric pressure, significantly high acoustic …
Computation Of Acoustic Ressure Fields Produced In Feline Brain By High-Intensity Focused Ultrasound, Nazanin Omidi
Computation Of Acoustic Ressure Fields Produced In Feline Brain By High-Intensity Focused Ultrasound, Nazanin Omidi
Electronic Theses and Dissertations
In 1975, Dunn et al. (Jasa 58:512-514) shothat a simple relation describes the ultrasonic threshold for cavitation induced changes in the mammalian brain. The thresholds for tissue damage were estimated for a variety of acoustic parameters in exposed feline brain. The goal of this study was to improve the estimates for acoustic pressures and intensities present in vivo during those experimental exposures by estimating them using nonlinear rather than linear theory. In our current project, the acoustic pressure waveforms produced in the brains of anesthetized felines were numerically simulated for a spherically focused, nominally f1-transducer (focal length = 13 cm) …