Digital Commons Network^™

Arctic Air Pollution: New Insights From Polarcat-Ipy, Katherine S. Law, Andreas Stohl, Patricia K. Quinn, Charles A. Brock, John F. Burkhart, Jean-Daniel Paris, Gerard Ancellet, Hanwant B. Singh, Anke Roiger, Hans Schlager, Jack E. Dibb, Daniel J. Jacob, S R. Arnold, Jacques Pelon, Jennie L. Thomas

Earth Sciences

Given the rapid nature of climate change occurring in the Arctic and the difficulty climate models have in quantitatively reproducing observed changes such as sea ice loss, it is important to improve understanding of the processes leading to climate change in this region, including the role of short-lived climate pollutants such as aerosols and ozone. It has long been known that pollution produced from emissions at midlatitudes can be transported to the Arctic, resulting in a winter/spring aerosol maximum known as Arctic haze. However, many uncertainties remain about the composition and origin of Arctic pollution throughout the troposphere; for example, …

Assessing Effects Of Permafrost Thaw On C Fluxes Based On Multiyear Modeling Across A Permafrost Thaw Gradient At Stordalen, Sweden, Jia Deng, C Li, Steve Frolking, Y Zhang, K Backstrand, P Crill

Earth Sciences

Northern peatlands in permafrost regions contain a large amount of organic carbon (C) in the soil. Climate warming and associated permafrost degradation are expected to have significant impacts on the C balance of these ecosystems, but the magnitude is uncertain. We incorporated a permafrost model, Northern Ecosystem Soil Temperature (NEST), into a biogeochemical model, DeNitrificationDeComposition (DNDC), to model C dynamics in highlatitude peatland ecosystems. The enhanced model was applied to assess effects of permafrost thaw on C fluxes of a subarctic peatland at Stordalen, Sweden. DNDC simulated soil freeze–thaw dynamics, net ecosystem exchange of CO2 (NEE), and CH4 fluxes across …

Water: Macro-Scale Process-Based Modeling Of Water, Steve Frolking, Richard B. Lammers, Danielle S. Grogan

Earth Sciences

No abstract provided.

Atmospheric Oxidation Chemistry And Ozone Production: Results From Sharp 2009 In Houston, Texas, Katherine A. Duderstadt, Jack E. Dibb, Charles H. Jackman, Cora E. Randall, Stanley C. Solomon, Michael J. Mills, Nathan A. Schwadron, Harlan E. Spence

Earth Sciences

This study considers whether spikes in nitrate in snow sampled at Summit, Greenland, from August 2000 to August 2002 are related to solar proton events. After identifying tropospheric sources of nitrate on the basis of correlations with sulfate, ammonium, sodium, and calcium, we use the three-dimensional global Whole Atmosphere Community Climate Model (WACCM) to examine unaccounted for nitrate spikes. Model calculations confirm that solar proton events significantly impact HOx, NOx, and O3 levels in the mesosphere and stratosphere during the weeks and months following the major 9 November 2000 solar proton event. However, solar proton event (SPE)-enhanced NOy calculated within …

Nitrate Deposition To Surface Snow At Summit, Greenland, Following The 9 November 2000 Solar Proton Event, Katherine A. Duderstadt, Jack E. Dibb, Charles H. Jackman, Cora E. Randall, Stanley C. Solomon, Michael J. Mills, Nathan A. Schwadron, Harlan E. Spence

Earth Sciences

Abstract

This study considers whether spikes in nitrate in snow sampled at Summit, Greenland, from August 2000 to August 2002 are related to solar proton events. After identifying tropospheric sources of nitrate on the basis of correlations with sulfate, ammonium, sodium, and calcium, we use the three-dimensional global Whole Atmosphere Community Climate Model (WACCM) to examine unaccounted for nitrate spikes. Model calculations confirm that solar proton events significantly impact HO_x, NO_x, and O₃ levels in the mesosphere and stratosphere during the weeks and months following the major 9 November 2000 solar proton event. However, solar …

Intercomparison Of Field Measurements Of Nitrous Acid (Hono) During The Sharp Campaign, J R. Pinto, Jack E. Dibb, B H. Lee, B Rappengluck, E C. Wood, M Levy, R Y. Zhang, Barry Lefer, Xinrong Ren, J Stutz, C Tsai, L Ackermann, J Golovko, S C. Herndon, M Oakes, Q Y. Meng, J W. Munger, M Zahniser, J Zheng

Earth Sciences

Because of the importance of HONO as a radical reservoir, consistent and accurate measurements of its concentration are needed. As part of SHARP (Study of Houston Atmospheric Radical Precursors), time series of HONO were obtained by six different measurement techniques on the roof of the Moody Tower at the University of Houston. Techniques used were long path differential optical absorption spectroscopy (DOAS), stripping coil-visible absorption photometry (SC-AP), long path absorption photometry (LOPAP® ), mist chamber/ion chromatography (MC-IC), quantum cascade-tunable infrared laser differential absorption spectroscopy (QC-TILDAS), and ion drift-chemical ionization mass spectrometry (ID-CIMS). Various combinations of techniques were in operation from …

Brown Carbon In The Continental Troposphere, Jiumeng Liu, Eric Scheuer, Jack E. Dibb, Luke D. Ziemba, Kenn L. Thornhill, Bruce Anderson, Armin Wisthaler, Tomas Mikoviny, J J. Devi, Mike Bergin, Rodney J. Weber

Earth Sciences

No abstract provided.

Mercury Speciation At A Coastal Site In The Northern Gulf Of Mexico: Results From The Grand Bay Intensive Studies In Summer 2010 And Spring 2011, Xinrong Ren, Winston T. Luke, Paul Kelley, Mark Cohen, Fong Ngan, Richard Artz, Jake Walker, Steve Brooks, Christopher Moore, Phil Swartzendruber, Dieter Bauer, James Remeika, Anthony Hynes, Jack E. Dibb, John Rolison, Nishanth Krishnamurthy, William M. Landing, Arsineh Hecobian, Jeffery Shook, L Gregory Huey

Earth Sciences

During two intensive studies in summer 2010 and spring 2011, measurements of mercury species including gaseous elemental mercury (GEM), gaseous oxidized mercury (GOM), and particulate-bound mercury (PBM), trace chemical species including O₃, SO₂, CO, NO, NO_Y, and black carbon, and meteorological parameters were made at an Atmospheric Mercury Network (AMNet) site at the Grand Bay National Estuarine Research Reserve (NERR) in Moss Point, Mississippi. Surface measurements indicate that the mean mercury concentrations were 1.42 ± 0.12 ng∙m⁻³ for GEM, 5.4 ± 10.2 pg∙m⁻³ for GOM, and 3.1 ± 1.9 pg∙m⁻³ for …

Mapping Crop Cycles In China Using Modis-Evi Time Series, Le Li, Mark A. Friedl, Qinchuan Xin, Josh M. Gray, Yaozhong Pan, Steve Frolking

Earth Sciences

As the Earth’s population continues to grow and demand for food increases, the need for improved and timely information related to the properties and dynamics of global agricultural systems is becoming increasingly important. Global land cover maps derived from satellite data provide indispensable information regarding the geographic distribution and areal extent of global croplands. However, land use information, such as cropping intensity (defined here as the number of cropping cycles per year), is not routinely available over large areas because mapping this information from remote sensing is challenging. In this study, we present a simple but efficient algorithm for automated …

Size And Frequency Of Natural Forest Disturbances And Amazon Carbon Balance, Fernando D.B. Espirito-Santo, Manuel Gloor, Michael Keller, Yadvinder Malhi, Sassan Saatchi, Bruce Nelson, Raimundo C. Oliveira Jr, Cleuton Pereira, Jon Lloyd, Steve Frolking, Michael W. Palace, Yosio E. Shimabukuro, Valdete Duarte, Abel Monteagudo Mendoza, Gabriela Lopez-Gonzalez, Tim R. Baker, Ted Feldpausch, Roel J.W. Brienen, Gregory P. Asner, Doreen S. Boyd, Oliver L. Phillips

Earth Sciences

Forest inventory studies in the Amazon indicate a large terrestrial carbon sink. However, field plots may fail to represent forest mortality processes at landscape-scales of tropical forests. Here we characterize the frequency distribution of disturbance events in natural forests from 0.01 ha to 2,651 ha size throughout Amazonia using a novel combination of forest inventory, airborne lidar and satellite remote sensing data. We find that small-scale mortality events are responsible for aboveground biomass losses of B1.28 Pg C y 1 over the entire Amazon region. We also find that intermediate-scale disturbances account for losses of B0.01 Pg C y 1 …

Representation Of Multiple Cropping Systems In Land Use Data Sets, K Waha, A Bondeau, Steve Frolking, F T. Portmann, S Siebert

Earth Sciences

No abstract provided.

Ice Cores From The St. Elias Mountains, Yukon, Canada: Their Significance For Climate, Atmospheric Composition And Volcanism In The North Pacific Region, Christian Zdanowicz, David Fisher, Jocelyne Bourgeois, Mike Demuth, James Zheng, Paul A. Mayewski, K Kreutz, Erich Osterberg, Kaplan Yalcin, Cameron P. Wake, Eric J. Steig, Duane Froese, Kumiko Goto-Azuma

Earth Sciences

A major achievement in research supported by the Kluane Lake Research Station was the recovery, in 2001 –02, of a suite of cores from the icefields of the central St. Elias Mountains, Yukon, by teams of researchers from Canada, the United States, and Japan. This project led to the development of parallel, long (103 – 104 year) ice-core records of climate and atmospheric change over an altitudinal range of more than 2 km, from the Eclipse Icefield (3017 m) to the ice-covered plateau of Mt. Logan (5340 m). These efforts built on earlier work recovering single ice cores in this …

Glaciers And Small Ice Caps In The Macro-Scale Hydrological Cycle: An Assessment Of Present Conditions And Future Changes, Richard B. Lammers, R Hock, Alexander Prusevich, A Bliss, V Radic, Stanley Glidden, Danielle S. Grogan, Steve Frolking

Earth Sciences

Glacier and small ice cap melt water contributions to the global hydrologic cycle are an important component of human water supply and for sea level rise. This melt water is used in many arid and semi-arid parts of the world for direct human consumption as well as indirect consumption by irrigation for crops, serving as frozen reservoirs of water that supplement runoff during warm and dry periods of summer when it is needed the most. Additionally, this melt water reaching the oceans represents a direct input to sea level rise and therefore accurate estimates of this contribution have profound economic …

Adaptability Of Irrigation To A Changing Monsoon In India: How Far Can We Go?, E Zaveri, Danielle S. Grogan, K Fisher-Vanden, Steve Frolking, D H. Wrenn

Earth Sciences

Agriculture and the monsoon are inextricably linked in India. A large part of the steady rise in agricultural production since the onset of the Green Revolution in the 1960’s has been attributed to irrigation. Irrigation is used to supplement and buffer crops against precipitation shocks, but water availability for such use is itself sensitive to the erratic, seasonal and spatially heterogeneous nature of the monsoon. Most attention in the literature is given to crop yields (Guiteras, 2009; Fishman, 2012; Auffhammer et al, 2011) and their ability to withstand precipitation shocks, in the presence of irrigation (Fishman, 2012). However, there remains …

Effect Of Carex Rostrata On Seasonal And Interannual Variability In Peatland Methane Emissions, Genevieve L. Noyce, Ruth Varner, Jill L. Bubier, Steve Frolking

Earth Sciences

Peatlands are a large natural source of atmospheric methane (CH₄), and the sedge Carex rostrata plays a critical role in the production, oxidation, and transport of CH₄ in these systems. This 4 year clipping experiment examined the changes in CH₄ emissions from a temperate peatland after removing all aboveground C. rostrata biomass. Methane fluxes, dissolved CH₄, and environmental variables were measured during spring, summer, and fall from 2008 to 2011. Clipping and removing the C. rostrata leaves and stems caused an immediate decrease in CH₄ emissions that persisted over 4 years of this …

In Situ Permafrost Thaw Due To Climate Change Drives Holistic Microbial Community Shifts With Implications For Methane Cycling, R Monday, C K. Mccalley, S B. Hodgkins, Virginia Rich, Steve Frolking, S R. Saleska, Andrew Barnes, J Chanton, P Crill

Earth Sciences

Thawing permafrost is a potentially significant source of radiative forcing feedback due to increased emissions of methane, a biogenic greenhouse gas (GHG). This study investigated changes in the microbial community along a permafrost thaw gradient at Stordalen Mire, Sweden using 16S rRNA gene amplicon and metagenomic methods. In situ measurements of geochemical parameters, including CH4 and C isotopes, enabled linkage of community dynamics to significant shifts in C balance. The thaw gradient ranged from intact at a palsa (low productivity and GHG emissions), through partially thawed in a bog (high productivity, low GHG emissions) to a completely thawed fen (high …