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Wet Deposition In A Global Size-Dependent Aerosol Transport Model: 2. Influence Of The Scavenging Scheme On 210pb Vertical Profiles, Surface Concentrations, And Deposition, W Guelle, Y J. Balkanski, Jack E. Dibb, M Schulz, F Dulac Nov 1998

Wet Deposition In A Global Size-Dependent Aerosol Transport Model: 2. Influence Of The Scavenging Scheme On 210pb Vertical Profiles, Surface Concentrations, And Deposition, W Guelle, Y J. Balkanski, Jack E. Dibb, M Schulz, F Dulac

Earth Sciences

The main atmospheric sink for submicron aerosols is wet removal. Lead 210, the radioactive decay product of 222Rn, attaches immediately after being formed to submicron particles. Here we compare the effects of three different wet-scavenging schemes used in global aerosol simulations on the 210Pb aerosol distribution using an off-line, size-resolved, global atmospheric transport model. We highlight the merits and shortcomings of each scavenging scheme at reproducing available measurements, which include concentrations in surface air and deposition, as well as vertical profiles observed over North America and western and central North Pacific. We show that model-measurement comparison of total …


Soluble Species In Aerosol And Snow And Their Relationship At Glacier 1, Tien Shan, China, Junying Sun, Dahe Qin, Paul A. Mayewski, Jack E. Dibb, Sallie I. Whitlow, Zhongqin Lee, Qinzhao Yang Nov 1998

Soluble Species In Aerosol And Snow And Their Relationship At Glacier 1, Tien Shan, China, Junying Sun, Dahe Qin, Paul A. Mayewski, Jack E. Dibb, Sallie I. Whitlow, Zhongqin Lee, Qinzhao Yang

Earth Sciences

Simultaneous sampling of aerosol (n = 20) and snow (n = 114) was made at Glacier 1, Tien Shan, between May 19 and June 29, 1996. Similar temporal patterns of some major ion (calcium, magnesium, potassium, sodium, chloride, and sulfate) concentrations between snow and aerosol show that snow chemistry basically reflects changes in the chemistry of the atmosphere. This gives us confidence in the reconstruction of past atmospheric change using some snow data. There are no significant correlations between aerosol and snow samples for ammonium and nitrate. This suggests that post-depositional and/or post-collection processes may alter ammonium and nitrate concentrations …


Nitric Acid Scavenging By Mineral And Biomass Burning Aerosols, A Tabazadeh, M Z. Jacobson, H B. Singh, O Brian Toon, J S. Lin, R B. Chatfield, A N. Thakur, R. Talbot, Jack E. Dibb Nov 1998

Nitric Acid Scavenging By Mineral And Biomass Burning Aerosols, A Tabazadeh, M Z. Jacobson, H B. Singh, O Brian Toon, J S. Lin, R B. Chatfield, A N. Thakur, R. Talbot, Jack E. Dibb

Earth Sciences

The abundance of gas phase nitric acid in the upper troposphere is overestimated by global chemistry-transport models, especially during the spring and summer seasons. Recent aircraft data obtained over the central US show that mineral aerosols were abundant in the upper troposphere during spring. Chemical reactions on mineral dust may provide an important sink for nitric acid. In regions where the mineral dust abundance is low in the upper troposphere similar HNO3 removal processes may occur on biomass burning aerosols. We propose that mineral and biomass burning aerosols may provide an important global sink for gas phase nitric acid, …


Influence Of Vertical Transport On Free Tropospheric Aerosols Over The Central Usa In Springtime, R. Talbot, Jack E. Dibb, M Loomis May 1998

Influence Of Vertical Transport On Free Tropospheric Aerosols Over The Central Usa In Springtime, R. Talbot, Jack E. Dibb, M Loomis

Earth Sciences

Measurements of the atmospheric aerosol chemical composition during the Subsonic Aircraft: Contrail and Cloud Effects Special Study (SUCCESS) indicate substantial vertical transport of boundary layer aerosol to the free troposphere over the south-central United States during springtime. Mixing ratios of water-soluble aerosol Ca 2+ at 6 - 12 km altitude exhibited a median mixing ratio of 20 pptv, with 15% of the measurements > 100 pptv and a maximum of ! 235 pptv. In air parcels with enhanced Ca 2+, the ratios K+/Ca 2+, Mg2+/Ca 2+, and Na+/Ca 2+ in the bulk aerosol were distinctly characteristic of those in limestone and/or …


Tropospheric Sulfate Distribution During Success: Contributions From Jet Exhaust And Surface Sources, Jack E. Dibb, R. Talbot, M Loomis May 1998

Tropospheric Sulfate Distribution During Success: Contributions From Jet Exhaust And Surface Sources, Jack E. Dibb, R. Talbot, M Loomis

Earth Sciences

The distribution of SO4= aerosol over the central US during SUCCESS indicates that surface sources of SO4= and SO2 in the western US caused SO4= enhancements up to 10 km altitude. The mean (median) SO4= mixing ratio in the mid- and upper-troposphere increased from 24 (16) pptv over the Pacific ocean to 58 (29) pptv over the central plains. Above 10 km the SO4=mixing ratio was essentially the same in both regions, and also when the geographic classifications were further partitioned into upper tropospheric and lower stratospheric categories …


Relationship Between Continuous Aerosol Measurements And Firn Core Chemistry Over A 10-Year Period At The South Pole, M H. Bergin, E A. Meyerson, Jack E. Dibb, Paul A. Mayewski Apr 1998

Relationship Between Continuous Aerosol Measurements And Firn Core Chemistry Over A 10-Year Period At The South Pole, M H. Bergin, E A. Meyerson, Jack E. Dibb, Paul A. Mayewski

Earth Sciences

Before ice core chemistry can be used to estimate past atmospheric chemistry it is necessary to establish an unambiguous link between concentrations of chemical species in the air and snow. For the first time a continuous long-term record of aerosol properties (aerosol light scattering coefficient, σsp, and Ångström exponent, å) at the South Pole are compared with the chemical record from a high resolution firn core (∼10 samples per year) covering the period from 1981 to 1991. Seasonal signals in å, associated with winter minima due to coarse mode seasalt and summer maxima due to accumulation mode sulfate …


Relationship Between Ecosystem Productivity And Photosynthetically-Active Radiation For Northern Peatlands, Steve Frolking, Jill L. Bubier, Tim R. Moore, T Ball, L M. Bellisario, A Bhardwaj, P Carroll, P Crill, P M. Lafleur, Harry Mccaughey, Nigel T. Roulet, Andrew E. Suyker, J M. Whittington, G J. Whiting Mar 1998

Relationship Between Ecosystem Productivity And Photosynthetically-Active Radiation For Northern Peatlands, Steve Frolking, Jill L. Bubier, Tim R. Moore, T Ball, L M. Bellisario, A Bhardwaj, P Carroll, P Crill, P M. Lafleur, Harry Mccaughey, Nigel T. Roulet, Andrew E. Suyker, J M. Whittington, G J. Whiting

Earth Sciences

We analyzed the relationship between net ecosystem exchange of carbon dioxide (NEE) and irradiance (as photosynthetic photon flux density or PPFD), using published and unpublished data that have been collected during midgrowing season for carbon balance studies at seven peatlands in North America and Europe. NEE measurements included both eddy-correlation tower and clear, static chamber methods, which gave very similar results. Data were analyzed by site, as aggregated data sets by peatland type (bog, poor fen, rich fen, and all fens) and as a single aggregated data set for all peatlands. In all cases, a fit with a rectangular hyperbola …


Air-Snow Exchange Of Hno3 And Noy At Summit, Greenland, Jack E. Dibb, R. Talbot, J W. Munger, Daniel J. Jacob, S M. Fan Feb 1998

Air-Snow Exchange Of Hno3 And Noy At Summit, Greenland, Jack E. Dibb, R. Talbot, J W. Munger, Daniel J. Jacob, S M. Fan

Earth Sciences

Ice core records of NO3 deposition to polar glaciers could provide unrivaled information on past photochemical status and N cycling dynamics of the troposphere, if the ice core records could be inverted to yield concentrations of reactive N oxides in the atmosphere at past times. Limited previous investigations at Summit, Greenland, have suggested that this inversion may be difficult, since the levels of HNO3 and aerosol-associated NO3 over the snow are very low in comparison with those of NO3 in the snow. In addition, it appears that some fraction of the NO3 …


Preservation Of Glaciochemical Time-Series In Snow And Ice From The Penny Ice Cap, Baffin Island, Nancy S. Grumet, Cameron P. Wake, Gregory A. Zielinski, David Fisher, Roy M. Koerner, John D. Jacobs Feb 1998

Preservation Of Glaciochemical Time-Series In Snow And Ice From The Penny Ice Cap, Baffin Island, Nancy S. Grumet, Cameron P. Wake, Gregory A. Zielinski, David Fisher, Roy M. Koerner, John D. Jacobs

Earth Sciences

A detailed investigation of major ion concentrations of snow and ice in the summit region of Penny Ice Cap (PIC) was performed to determine the effects of summer melt on the glaciochemical time-series. While ion migration due to meltwater percolation makes it difficult to confidently count annual layers in the glaciochemical profiles, time-series of these parameters do show good structure and a strong one year spectral component, suggesting that annual to biannual signals are preserved in PIC glaciochemical records.


Characteristics Of Modern Atmospheric Dust Deposition In Snow On The Penny Ice Cap, Baffin Island, Arctic Canada, Christian Zdanowicz, Gregory A. Zielinski, Cameron P. Wake Jan 1998

Characteristics Of Modern Atmospheric Dust Deposition In Snow On The Penny Ice Cap, Baffin Island, Arctic Canada, Christian Zdanowicz, Gregory A. Zielinski, Cameron P. Wake

Earth Sciences

We evaluated the concentration, size and distribution of insoluble dust microparticles in snowpits on the Penny Ice Cap (PIC), Baffin Island, to define (1) the characteristics of modern atmospheric dust deposition at the site, (2) the relative contributions of proximal and distal dust sources, and (3) the effects of summer melting on depositional signals in snow. The mean concentration (143 mg kg−1), flux (4.8 mg cm2 yr−1) and diameter (2.3 mm) of dust deposited on the PIC are similar to those observed in remote Arctic sites such as central Greenland, implying that dust is primarily supplied through long-range transport from …


The Pursuit Of Isotopic And Molecular Fire Tracers In The Polar Atmosphere And Cryosphere, L A. Currie, Jack E. Dibb, G A. Klouda, B A. Benner Jr., J M. Conny, S R. Biegalski, D B. Klinedinst, D R. Cahoon, N C. Hsu Jan 1998

The Pursuit Of Isotopic And Molecular Fire Tracers In The Polar Atmosphere And Cryosphere, L A. Currie, Jack E. Dibb, G A. Klouda, B A. Benner Jr., J M. Conny, S R. Biegalski, D B. Klinedinst, D R. Cahoon, N C. Hsu

Earth Sciences

We present an overview of recent multidisciplinary, multi-institutional efforts to identify and date major sources of combustion aerosol in the current and paleoatmospheres. The work was stimulated, in part, by an atmospheric particle 'sample of opportunity' collected at Summit, Greenland in August 1994, that bore the 14C imprint of biomass burning. During the summer field seasons of 1995 and 1996, we collected air filter, surface snow and snowpit samples to investigate chemical and isotopic evidence of combustion particles that had been transported from distant fires. Among the chemical tracers employed for source identification are organic acids, potassium and ammonium ions, …