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Coupled Simulation Of Dnapl Infiltration And Dissolution In Three-Dimensional Heterogeneous Domains: Process Model Validation, Amalia Kokkinaki, D M. O'Carroll, C J. Werth, B E. Sleep
Coupled Simulation Of Dnapl Infiltration And Dissolution In Three-Dimensional Heterogeneous Domains: Process Model Validation, Amalia Kokkinaki, D M. O'Carroll, C J. Werth, B E. Sleep
Environmental Science
A three-dimensional multiphase numerical model was used to simulate the infiltration and dissolution of a dense nonaqueous phase liquid (DNAPL) release in two experimental flow cells containing different heterogeneous and well-characterized permeability fields. DNAPL infiltration was modeled using Brooks-Corey-Burdine hysteretic constitutive relationships. DNAPL dissolution was simulated using a rate-limited mass transfer expression with a velocity-dependent mass transfer coefficient and a thermodynamically based calculation of DNAPL-water interfacial area. The model did not require calibration of any parameters. The model predictions were compared to experimental measurements of high-resolution DNAPL saturations and effluent concentrations. The predicted concentrations were in close agreement with measurements …