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Airborne Measurements Of Carbonaceous Aerosol Soluble In Water Over Northeastern United States: Method Development And An Investigation Into Water-Soluble Organic Carbon Sources, A. P. Sullivan, Richard E. Peltier, C. A. Brock, J. A. De Gouw, J. S. Holloway, C. Warneke, A. G. Wollny, R. J. Weber
Airborne Measurements Of Carbonaceous Aerosol Soluble In Water Over Northeastern United States: Method Development And An Investigation Into Water-Soluble Organic Carbon Sources, A. P. Sullivan, Richard E. Peltier, C. A. Brock, J. A. De Gouw, J. S. Holloway, C. Warneke, A. G. Wollny, R. J. Weber
Richard E. Peltier
A particle-into-liquid sampler (PILS) was coupled to a total organic carbon (TOC) analyzer for 3 s integrated measurements of water-soluble organic carbon (WSOC) in PM1 ambient particles. The components of the instrument are described in detail. The PILS-TOC was deployed on the NOAA WP-3D aircraft during the NEAQS/ITCT 2004 program to investigate WSOC sources over the northeastern United States and Canada. Two main sources were identified: biomass burning emissions from fires in Alaska and northwestern Canada and emissions emanating from urban centers. Biomass burning WSOC was correlated with carbon monoxide (CO) and acetonitrile (r2 > 0.88). These plumes were intercepted in …
Concentrations And Sources Of Organic Carbon Aerosols In The Free Troposphere Over North America, Colette L. Heald, Daniel J. Jacob, Solène Turquety, Rynda C. Hudman, Rodney J. Weber, Amy P. Sullivan, Richard E. Peltier, Eliot L. Atlas, Joost A. De Gouw, Carsten Warneke, John S. Holloway, J. Andrew Neuman, John H. Seinfeld, Frank M. Flocke
Concentrations And Sources Of Organic Carbon Aerosols In The Free Troposphere Over North America, Colette L. Heald, Daniel J. Jacob, Solène Turquety, Rynda C. Hudman, Rodney J. Weber, Amy P. Sullivan, Richard E. Peltier, Eliot L. Atlas, Joost A. De Gouw, Carsten Warneke, John S. Holloway, J. Andrew Neuman, John H. Seinfeld, Frank M. Flocke
Richard E. Peltier
Aircraft measurements of water-soluble organic carbon (WSOC) aerosol over NE North America during summer 2004 (ITCT-2K4) are simulated with a global chemical transport model (GEOS-Chem) to test our understanding of the sources of organic carbon (OC) aerosol in the free troposphere (FT). Elevated concentrations were observed in plumes from boreal fires in Alaska and Canada. WSOC aerosol concentrations outside of these plumes average 0.9 ± 0.9 mg C m 3 in the FT (2–6 km). The corresponding model value is 0.7 ± 0.6 mg C m 3, including 42% from biomass burning, 36% from biogenic secondary organic aerosol (SOA), and …
Single-Particle Mass Spectrometry Of Tropospheric Aerosol Particles, D. M. Murphy, D. J. Cziczo, K. D. Froyd, P. K. Hudson, B. M. Matthew, A. M. Middlebrook, Richard E. Peltier, A. Sullivan, D. S. Thomson, R. J. Weber
Single-Particle Mass Spectrometry Of Tropospheric Aerosol Particles, D. M. Murphy, D. J. Cziczo, K. D. Froyd, P. K. Hudson, B. M. Matthew, A. M. Middlebrook, Richard E. Peltier, A. Sullivan, D. S. Thomson, R. J. Weber
Richard E. Peltier
The Particle Analysis by Laser Mass Spectrometry (PALMS) instrument has measured the composition of single particles during a number of airborne and ground-based campaigns. In the regions studied, 30% to over 80% of the aerosol mass in the free troposphere was carbonaceous material. Most of this carbonaceous material was probably organic. Although there were variations in their amounts, over 90% of accumulation mode particles away from local sources were internal mixtures of sulfates and carbonaceous material. Within this internal mixing, there was variation in the pattern of carbonaceous peaks in the spectra, especially in peaks related to organic acids. Particles …