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Articles 1 - 30 of 79
Full-Text Articles in Entire DC Network
Model Fe(Iii) Porphyrin Systems: Axial Ligation In Oxidized Cytochrome P-450.S, G. C. Papaefthymiou, Richard B. Frankel, S. Foner, S. C. Tang, S. Koch, R. H. Holm
Model Fe(Iii) Porphyrin Systems: Axial Ligation In Oxidized Cytochrome P-450.S, G. C. Papaefthymiou, Richard B. Frankel, S. Foner, S. C. Tang, S. Koch, R. H. Holm
Physics
In an effort to develop useful experimental criteria to distinguish among the viable axial ligation possibilities of O, N, and S coordination in oxidized cytochrome P-450. S (substrate-bound, high-spin), syntheticmodel compounds with O-(Fe(PPIXDME) (OEt) and Fe(PPIXDME) (OC6H4NO2)) and S-(Fe(PPIXDME) (S6H4NO2) and Fe(OEP) (SPh)) donor axial ligands were prepared and studied by Mössbauer spectroscopy. Ferric hemoglobin and myoglobin were used as model compounds with N-axial coordination. The isomer shifts (δ) and quadrupole splittings (ΔEQ) observed are typical of high-spin Fe(III) porphyrins and are comparable with results …
Synthetic Analogs Of The Active Sites Of Oxidized And Reduced Rubredoxin, Richard B. Frankel, G. C. Papaefthymiou, R. W. Lane, R. H. Holm
Synthetic Analogs Of The Active Sites Of Oxidized And Reduced Rubredoxin, Richard B. Frankel, G. C. Papaefthymiou, R. W. Lane, R. H. Holm
Physics
The bischelate monoanion [Fe((SCH2)2C6H4)2]1- contains an unconstrained, near-tetrahedral Fe(III)-S4 coordination unit (similar to the Fe-S4 coordinationunit occurring in rubredoxin proteins) and exhibits the Fe(III)/Fe(II) redox couple. Mossbauer parameters at 77 K are isomer shift δ = 0.13 mm/s (relative to iron metal) and electric quadrupole splitting ΔEQ = 0.57 mm/s. Application of an external magnetic field parallel to the direction of observation at 4.2 K induces a saturation magnetic hyperfine field of - 380 kOe. Upon reduction to the dianion [Fe((SCH2)2C …
Experiments On The Attenuation Of Third Sound In Saturated Superfluid Helium Films, Robert Hallock, K. L. Telschow, R. K. Galkiewicz
Experiments On The Attenuation Of Third Sound In Saturated Superfluid Helium Films, Robert Hallock, K. L. Telschow, R. K. Galkiewicz
Robert Hallock
Upper limits of the attenuation of third sound in saturated superfluid 4He films have been measured in three separate experiments. Our observations at frequencies from 0.1 to 200 Hz indicate that the attenuation in these thick films is substantially lower than would be inferred from the only previous experiment done on saturated films. We observe the third-sound velocity to have the temperature dependence predicted by Bergman.
Review Of Quantum States Of Atoms, Molecules And Solids, M. Eugene Rudd
Review Of Quantum States Of Atoms, Molecules And Solids, M. Eugene Rudd
M. Eugene Rudd Publications
The subjects of atomic, molecular and solid-state physics have only rarely been treated at an advanced level in a single volume. The notable exception, of course, is John C. Slater’s Quantum Theory of Matter. In the present book the three authors, Michael Morrison, Thomas Estle and Neal Lane, stress the unity among these fields by ernphasizing the concept of electronic quantum states in atoms, diatomic molecules and crystalline solids. Such a combination should be of basic interest to students in a variety of scientific fields and also form the basis for more advanced work in those three subjects themselves. …
Ultraviolet Stimulated Thermoluminescent Response Characteristics Of Aluminum Oxide, Edward Ryan Iii
Ultraviolet Stimulated Thermoluminescent Response Characteristics Of Aluminum Oxide, Edward Ryan Iii
Masters Theses & Specialist Projects
This investigation has demonstrated that some aluminum oxide crystals have high sensitivity and are well suited for detecting and measuring ultraviolet radiation rates significantly less than .01 µW/cm2.
The thermoluminescent glow curve, linearity of response, and fading of the crystals were determined. An action spectrum was performed to determine the relative sensitivities of several crystals in a range of wavelengths from 230 nm to 546 nm.
The sensitivity of the crystals was found to decrease as a function of exposure. \n explanation for the decrease in sensitivity due to the presence of high temperature traps is presented.
This …
Ultraviolet Stimulated Thermoluminescent Response Characteristics Of Aluminum Oxide, Edward Ryan
Ultraviolet Stimulated Thermoluminescent Response Characteristics Of Aluminum Oxide, Edward Ryan
Masters Theses & Specialist Projects
This investigation has demonstrated that some aluminum oxide crystals have high sensitivity and are well suited for detecting and measuring ultraviolet radiation rates significantly less than 0.1 pW/cm2. The thermoluminescent glow curve, linearity of response, and fading of the crystals were determined. An action spectrum was performed to determine the relative sensitivities of several crystals in a range of wavelengths from 230 nm to 546 nm. The sensitivity of the crystals was found to decrease as a function of exposure. An explanation for the decrease in sensitivity due to the presence of high temperature traps is presented. This investigation has …
Energy Dependence Of Amorphizing Implant Dose In Silicon, John R. Dennis, Edward Boyd Hale
Energy Dependence Of Amorphizing Implant Dose In Silicon, John R. Dennis, Edward Boyd Hale
Physics Faculty Research & Creative Works
The radiation-induced transformation from crystalline to amorphous silicon was studied using ion implantation. The ion energy was varied from 20 to 180 keV for Li+, N+, Ne+, Ar+, and Kr +. The energy dependence of the critical amorphizing dose was determined by electron spin resonance. Comparison of the data with theoretical calculations of the energy density deposited into atomic processes showed good agreement. This energy-dependent agreement gave evidence that energy density is important to the transformation at both low and high implantation temperatures.
Computer Model Of A Fast Toroidal Plasma Compression, With Application To The Topolotron, H. Mark Nelson, Keith H. Brown, Charles A. Hart
Computer Model Of A Fast Toroidal Plasma Compression, With Application To The Topolotron, H. Mark Nelson, Keith H. Brown, Charles A. Hart
Faculty Publications
The method is developed for a comuputer sequence which models a fast toroidal theta or screw pinch for a highly conducting axially symmetric plasma. The computer sequence takes into account the self-inductances of the plasma and the external conductors which drive the compression as well as the mutual inductance which electromagnetically couples the two. The computer sequence is divided into three phases: a snowplow compression phase, an adiabatic compression phase, and a crowbarred circuit phase. The computer sequence is applied to a topolotron and an example is given of a magnetohydrodynamic equilibrium geometry for which the plasma surface possesses an …
Electron Transmission Studies Of The Negative Ion States Of Substituted Benzenes In The Gas Phase, Kenneth D. Jordan, J.A. Michejda, Paul Burrow
Electron Transmission Studies Of The Negative Ion States Of Substituted Benzenes In The Gas Phase, Kenneth D. Jordan, J.A. Michejda, Paul Burrow
Paul Burrow Publications
Temporary negative ions of benzene, aniline, phenol, anisole, fluoro-, chloro-, and bromobenzene, formed in the gas phase by capture of electrons into the low-lying π* orbitals, are studied by means of electron transmission spectroscopy. The electron affinities are determined and their relative values are interpreted in terms of resonance and inductive effects.
Excitation Of The N=2 State Of Atomic Hydrogen By Electron Impact In The Distorted-Wave Approximation, Ralph V. Calhoun, Don H. Madison, W. Neil Shelton
Excitation Of The N=2 State Of Atomic Hydrogen By Electron Impact In The Distorted-Wave Approximation, Ralph V. Calhoun, Don H. Madison, W. Neil Shelton
Physics Faculty Research & Creative Works
The differential cross sections for excitation of the n=2 state of atomic hydrogen by the impact of electrons with energies of 54, 100, 136, and 200 eV are calculated in the distorted-wave approximation with exchange included. Cross sections for excitation of the 2s1/2, 2p1/2, and 2p3/2 states are calculated and summed to give the n=2 differential cross sections. The results of this calculation are compared with previous theoretical calculations and with recent absolute experimental data.
Abstract: Mössbauer Spectroscopy Of Pdh Fe Alloys, M. Weber, C. R. Abeledo, Richard B. Frankel, Brian B. Schwartz
Abstract: Mössbauer Spectroscopy Of Pdh Fe Alloys, M. Weber, C. R. Abeledo, Richard B. Frankel, Brian B. Schwartz
Physics
Large changes in the electron susceptibility of PdH alloys have been observed with increasing H concentration, with important consequences for the magnetic and superconducting properties of these alloys. (1) To observe the effect of the changing spin susceptibility, we have studied PdH Fe alloys with 2, 1 and < 0.1 at. % Fe by Mössbauer spectroscopy in external magnetic fields. Mydosh (2) has reported spin glass behavior in the high Fe concentration alloys and Kondo phenomena in the dilute Fe alloys. For hydrogen-metal ratios < 0.5, α and β phases, with low and high hydrogen content respectively, coexist. For temperatures below Tc of the α phase but above Tc of the β phase, we observe a superposition of a six line spectrum and a single line corresponding to the α and β phases respectively. (3) In an applied field, the β phase magnetizes and both phases have hyperfine fields which extrapolate to …
Mössbauer And Nmr Studies Of Site Substitution And Magnetic Structure Of Fe3-XMnXSi Alloys, K. Raj, V. Niculescu, T. J. Burch, J. I. Budnick, Richard B. Frankel
Mössbauer And Nmr Studies Of Site Substitution And Magnetic Structure Of Fe3-XMnXSi Alloys, K. Raj, V. Niculescu, T. J. Burch, J. I. Budnick, Richard B. Frankel
Physics
The NMR measurements in Fe3−xMnxSi alloys show increasingly complex spectra for x > 0.75 due to overlapping signals from Fe, Si and Mn nuclei in various sites. Mössbauer experiments were undertaken to identify the Fe57 resonances. The combined NMR and Mössbauer results have been used to elucidate the site substitution and magnetic structure of these alloys for (0 < x < 1.75).
A Comparison Of The Rough Sphere Rotational Diffusion Model With Experimental Results For Liquid Methyl Iodide, Dane R. Jones, Scott L. Whittenburg, C. H. Wang
A Comparison Of The Rough Sphere Rotational Diffusion Model With Experimental Results For Liquid Methyl Iodide, Dane R. Jones, Scott L. Whittenburg, C. H. Wang
Chemistry and Biochemistry Faculty Publications
No abstract available.
Electronic And Magnetic Properties Of Amorphous And Crystalline Zr40Cu60-XFeX Alloys, F.R. Szofran, G.R. Gruzalski, John W. Weymouth, David J. Sellmyer, B.C. Giessen
Electronic And Magnetic Properties Of Amorphous And Crystalline Zr40Cu60-XFeX Alloys, F.R. Szofran, G.R. Gruzalski, John W. Weymouth, David J. Sellmyer, B.C. Giessen
David Sellmyer Publications
Electronic states and localized magnetic moments and their interactions were studied in amorphous and crystalline Zr40Cu60-xFex alloys for 0≤x≤12. Electrical resistivity, magnetic susceptibility, and high-field magnetization measurements were performed. In the dilute crystalline alloys Curie-Weiss behavior is seen in the susceptibility and is associated with localized moments (μeff≈3μB) on the iron atoms. At higher iron concentrations ferromagnetism is observed. Curie-Weiss behavior also is seen in the susceptibility of the dilute (0eff≈0.7μB). There is some evidence that the local environment of the Fe atoms is important and may depend …
Calculated Temperature Of Grid Lateral Wires In Microwave Power Triodes, Jewell Tucker
Calculated Temperature Of Grid Lateral Wires In Microwave Power Triodes, Jewell Tucker
Masters Theses & Specialist Projects
In microwave power triodes the grid drive power causes grid lateral wire heating. This development calculates the temperature of the wire as a function of the drive power, physical dimensions and characteristics of the wire material, for the following boundary conditions:
I. Constant grid drive, grid lateral wire of infinite length not connected to a heat sink.
II. Same as I except the wire is of finite length brazed to a grid frame.
III. The grid excitation in the form of pulses, and the grid lateral wire of finite length brazed to a grid frame.
the equations were verified experimentally …
Behavior Of A Manganin Coil At Elevated Temperatures And Pressures, Jonathan D. Weiss, Daniel L. Decker, H. B. Vanfleet
Behavior Of A Manganin Coil At Elevated Temperatures And Pressures, Jonathan D. Weiss, Daniel L. Decker, H. B. Vanfleet
Faculty Publications
We have determined the temperature dependence in the first-order pressure coefficient of a manganin coil to be dBetaB/dT= (4.2±0.8) ×10^-7 (kbar degrees C)^-1 in the equation R (T,P) =R (T,0)(1+BetaP+GammaP2), where R (T,P) is the coil resistance at temperature T and pressure P. The measurements were performed by simultaneously measuring the coil resistance and temperature at the transitions of mercury and bismuth, which were observed by differential thermal analysis.
Supralinearity Of Thermoluminescent Dosimeters, Leif Larsson, Robert Katz
Supralinearity Of Thermoluminescent Dosimeters, Leif Larsson, Robert Katz
Robert Katz Publications
The supralinear response of thermoluminescent dosimeters (TLDs) after irradiation with gamma- or beta-rays can be decomposed by use of the cumulative Poisson distribution into a sum of 1-or-more and 2-or-more hit components, suggesting the coexistence of both types of trap structures. Following the response of other 1-hit detectors, and of biological cells to energetic heavy ions, we expect and find that the supralinear response tends to disappear with alpha particle, and with neutron irradiation, and that the supralinear, or 2-hit, component tends to be more responsive to high LET (Linear Energy Transfer) radiations. Since the response of biological cells to …
The Quantum Defect Theory Approach, Anthony F. Starace
The Quantum Defect Theory Approach, Anthony F. Starace
Anthony F. Starace Publications
The Quantum Defect Theory (QDT) is a method of using the analytically known properties of excited electrons moving in a pure Coulomb field to describe atomic photoabsorption and electron-ion scattering processes in terms of a few parameters. These parameters may be determined either from experimental data or from ab initio theoretical calculations. In addition, they are usually nearly independent of energy in the threshold energy region (i.e., within a few eV of the atomic ionization threshold). Thus the determination of these parameters at any single energy suffices to predict the variation with energy of numerous atomic properties in the threshold …
18th Annual Rocky Mountain Spectroscopy Conference
18th Annual Rocky Mountain Spectroscopy Conference
Rocky Mountain Conference on Magnetic Resonance
Final program and abstracts from the 18th annual meeting of the Rocky Mountain Spectroscopy Conference, sponsored by the Rocky Mountain Section of the Society for Applied Spectroscopy. Held in Denver, Colorado, August 2-3, 1976.
Cross Sections For Excitation Of Atomic Hydrogen To The N=2, 3, And 4 States By 15-200-Kev Protons, John T. Park, Judith E. Aldag, Jacob M. George, Jerry Peacher
Cross Sections For Excitation Of Atomic Hydrogen To The N=2, 3, And 4 States By 15-200-Kev Protons, John T. Park, Judith E. Aldag, Jacob M. George, Jerry Peacher
Physics Faculty Research & Creative Works
Cross sections for the processes H++H(1 s)H++H*(n = 2, 3, 4) have been extracted from the energy-loss spectra of 15- to 200-keV protons by using a spectrum-fitting technique. Absolute cross sections have been obtained by normalization of the spectra to the theoretical cross section through the use of the Born approximation at 200 keV. The cross-section curves are very similar in shape with maxima at 60 keV. The results have been compared with available theoretical calculations. The n = 2 and n = 3 cross-section measurements are in very good agreement in curve shape with Glauber-approximation …
Electrical Conductivity Of Thin Lecithin-Cholesterol Membranes Due To 2,4-D, 2,4-Db, 2,4,5-T And 2,4-Dcp, Malkanthi Paulis
Electrical Conductivity Of Thin Lecithin-Cholesterol Membranes Due To 2,4-D, 2,4-Db, 2,4,5-T And 2,4-Dcp, Malkanthi Paulis
Dissertations and Theses
The effect of the following pesticides on DC electrical conductivity of lecithin-cholesterol membranes has been studied: endothall, paraquat, diquat, 2,4-D, 2,4-DB, 2,4,5-T, 2,4-DCP. It has been found that the ions of endothall, paraquat and diquat are essentially membrane impermeable and that they do not bind to the membrane surface. In contrast, 2,4-D, 2,4-DB, 2,4,5-T and 2,4-DCP induce electrical conductivity in lecithincholesterol membranes and in addition they also cause an increase in the nonactin-K+ membrane conductivity.
The compounds 2,4-D, 2,4-DB, 2,4,5-T and 2,4-DCP basically behave as class II uncouplers. The kinetic scheme of charge transfer across the membrane, based on …
Frequency-Mixing Detection (Fmd) Of Polarization-Modulated Light, R. M.A. Azzam
Frequency-Mixing Detection (Fmd) Of Polarization-Modulated Light, R. M.A. Azzam
Electrical Engineering Faculty Publications
When a light beam whose polarization and intensity are weakly modulated at a frequency ωm passes through a periodic analyzer of frequency ωa(<ωm) and the transmitted flux is linearly detected, the resulting total signal St consists of two components: (i) a periodic baseband signal Sbb with harmonics of frequencies nωa (n = 0,1,2,…) and (ii) an amplitude-modulated-carrier signal δSmc with center (carrier) frequency ωm and sideband frequencies at ωm ± nωa(n = 1,2,…). In this paper we show that the average polarization of the beam is determined …ω
Systematic Evaluation Of Cellular Radiosensitivity Parameters, R. A. Roth, S. C. Sharma, Robert Katz
Systematic Evaluation Of Cellular Radiosensitivity Parameters, R. A. Roth, S. C. Sharma, Robert Katz
Robert Katz Publications
Cellular radiosensitivity parameters of the track structure theory of Katz and co-workers are evaluated from a sum of squares minimizing computer program for nonlinear models. Based on these observations, suggestions are presented for efficient experiment design for the determination of these parameters from track-segment bombardments of high LET radiations.
Comparison Of Experimental And Theoretical Electron Ejection Cross Sections In Helium By Proton Impact From 5 To 100 Kev, M. Eugene Rudd, Don H. Madison
Comparison Of Experimental And Theoretical Electron Ejection Cross Sections In Helium By Proton Impact From 5 To 100 Kev, M. Eugene Rudd, Don H. Madison
Physics Faculty Research & Creative Works
Absolute values of doubly differential cross sections are obtained for electron production in helium by 5- to 100-keV proton impact. The measured values along with earlier data at higher energies are compared with theoretical plane-wave Born-approximation functions obtained from a Hartree-Fock potential. Not only is good agreement obtained at high impact energies (above 300 keV), but fairly good agreement is found at low energies (below about 20 keV). For electrons ejected in the backward hemisphere, unexpectedly poor agreement is noted at intermediate energies where the measured cross sections dip to 50% of the calculated values in some cases. Singly differential …
Modulated Generalized Ellipsometry, R. M.A. Azzam
Modulated Generalized Ellipsometry, R. M.A. Azzam
Electrical Engineering Faculty Publications
We extend ellipsometry to the direct measurement of small perturbations of the Jones matrix of any linear nondepolarizing optical sample (system) subjected to a modulating stimulus such as temperature, stress, or electric or magnetic field. The methodology of this technique, to be called Modulated Generalized Ellipsometry (MGE), is presented. First an ellipsometer with arbitrary polarizing and analyzing optics is assumed, and subsequently the discussion is specialized to a conventional ellipsometer having either the polarizer-sample-analyzer (PSA) or the polarizer-compensator-sample-analyzer (PCSA) arrangement. MGE provides the tool for the systematic study of thermo-optical, piezo-optical, electro-optical, magneto-optical, and other allied effects for both isotropic …
Observation Of Vibrationally Excited Nitrogen With A Simplified Electron Transmission Apparatus, J.A. Michejda, Paul Burrow
Observation Of Vibrationally Excited Nitrogen With A Simplified Electron Transmission Apparatus, J.A. Michejda, Paul Burrow
Paul Burrow Publications
A simple electron transmission apparatus is used to observe vibrationally excited N2 in the first two vibrational levels. The method is based on the pronounced peaks appearing in the total electron scattering cross section in the range of energy 2–4 eV. Because of the wide spacing between these peaks, good energy resolution is not required and measurements can be performed without an electron monochromator.
Reply To “Comments On ‘Theoretical Study Of Impurity-Induced First-Order Raman Spectra For The Alkali Halides’”, John R. Hardy, Arnold Karo
Reply To “Comments On ‘Theoretical Study Of Impurity-Induced First-Order Raman Spectra For The Alkali Halides’”, John R. Hardy, Arnold Karo
John R. Hardy Papers
This is a reply to the preceding comment by Page on the relative merits of the breathing-shell and deformation-dipole models for predicting defect-activated first-order Raman spectra. We show that when both models are parametrized in the same fashion the agreement between theory and experiment is comparable.
Metamagnetism In Single Crystal Γ-Co(Pyridine)2Cl2, S. Foner, Richard B. Frankel, W. M. Reiff, H. Wong, Gary J. Long
Metamagnetism In Single Crystal Γ-Co(Pyridine)2Cl2, S. Foner, Richard B. Frankel, W. M. Reiff, H. Wong, Gary J. Long
Physics
Small (≤1 mg) single crystals of γ-Co(pyr)2Cl2 have been grown and measurements of magnetic moment vs applied field H and temperature have been made for 0≤H≤54 kG and 1.25 K≤T≤4.2 K. At 1.25 K, metamagnetic transitions are observed along the a-axis at ~700 G; along the b-axis at both ~800 and ~1500 G; and along the c-axis at ~4 kG. The low field susceptibilities show a maximum at T≃3.4 K for each orientation. Magnetic saturation is not achieved at 54 kG; about 2.5 µB is achieved along the a*- or b-axes, whereas a lower moment is …
Hyperfine Interactions In Antiferromagnetic Eute Using The Te-125 Mossbauer Resonance, N. A. Blum, Richard B. Frankel
Hyperfine Interactions In Antiferromagnetic Eute Using The Te-125 Mossbauer Resonance, N. A. Blum, Richard B. Frankel
Physics
Europium telluride crystallizes in the NaCl structure and is antiferromagnetic with a Néel temperature TN of 9.6 K. We have used the 35.5 keV Møssbauer transition in Te-125 to examine the nature of the spontaneous magnetic moment which has been observed in conducting samples below TN. At 80 K the Mössbauer resonance spectrum consisted of a single absorption line comparable in width with the spectrum of nonmagnetic cubic ZnTe, indicating the absence of a significant quadrupole splitting at this temperature. At 4.2 K the line-width increased by a factor of 1.5, which is equivalent to a single magnetic hyperfine field …
Photoinization Cross Sections For Atomic Chlorine Using An Open-Shell Random-Phase Approximation, Anthony F. Starace, Lloyd Armstrong Jr.
Photoinization Cross Sections For Atomic Chlorine Using An Open-Shell Random-Phase Approximation, Anthony F. Starace, Lloyd Armstrong Jr.
Anthony F. Starace Publications
The use of the random-phase approximation with exchange (RPAE) for calculating partial and total photoionization cross sections and photoelectron angular distributions for open-shell atoms is examined for atomic chlorine. Whereas the RPAE corrections in argon (Z=18) are large, we find those in chlorine (Z=17) to be much smaller due to geometric factors. Hartree-Fock calculations with and without core relaxation are also presented. Sizable deviations from the close-coupling results of Conneely are found.