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Harmonic Generation Spectroscopy With A Two-Colour Laser Field Having Orthogonal Linear Polarizations, T. S. Sarantseva, M. V. Frolov, N. L. Manakov, M. Yu. Ivanov, Anthony F. Starace

Anthony F. Starace Publications

The interpretation of many high-order harmonic generation (HHG) experiments is based on the assumption that the HHG yield of an atom can be factorized into (i) a laser-dependent ‘electron wave packet’ with rather simple properties, including a nearly universal shape, and (ii) an atomic photorecombination cross section. We show that this factorization is restricted to linearly polarized laser fields and fails in two-colour laser fields with orthogonal polarizations. At the same time, we show how two-colour HHG spectroscopy using orthogonally polarized intense fundamental and relatively weak second harmonic fields makes a complete experiment possible that enables the retrieval of the …