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Gold Nanoparticle Generation Using In Situ Reduction On A Photoresist Polymer Substrate, Christopher J. Clukay
Gold Nanoparticle Generation Using In Situ Reduction On A Photoresist Polymer Substrate, Christopher J. Clukay
HIM 1990-2015
This report presents evidence that in-situ reduction of metal ions bound to a cross-linked polymer surface does not always result in nanoparticle formation solely at the interface, as is commonly assumed, but also as much as 40 nm deep within the polymer matrix. Tetrachloroaurate ions were bound using a variety of multi-functional amines to cured films of SU-8 -- a cross-linkable epoxide frequently used for micro- and nanofabrication -- and then treated using one of several reducing agents. The resulting gold-nanoparticle decorated films were examined by X-ray photoelectron spectroscopy and by plan-view and cross-sectional transmission electron microscopy. Reduction using sodium …
Approximation By Bernstein Polynomials At The Point Of Discontinuity, Jie Ling Liang
Approximation By Bernstein Polynomials At The Point Of Discontinuity, Jie Ling Liang
HIM 1990-2015
Chlodovsky showed that if x0 is a point of discontinuity of the first kind of the function f, then the Bernstein polynomials Bn(f, x0) converge to the average of the one-sided limits on the right and on the left of the function f at the point x0. In 2009, Telyakovskii in (5) extended the asymptotic formulas for the deviations of the Bernstein polynomials from the differentiable functions at the first-kind discontinuity points of the highest derivatives of even order and demonstrated the same result fails for the odd order case. Then in 2010, Tonkov in (6) found the right formulation …
Small-Scale Hybrid Alternative Energy Maximizer For Wind Turbines And Photovoltaic Panels, Ross Kerley
Small-Scale Hybrid Alternative Energy Maximizer For Wind Turbines And Photovoltaic Panels, Ross Kerley
HIM 1990-2015
This thesis describes the creation of a small-scale Hybrid Power System (HPS) that maximizes energy from a wind turbine and photovoltaic array. Small-scale HPS are becoming an increasingly viable energy solution as fossil fuel prices rise and more electricity is needed in remote areas. Modern HPS typically employ wind speed sensors and three power stages to extract maximum power. Modern systems also use passive rectifiers to convert AC from the wind turbine to DC that is usable by power electronics. This passive system inefficiently wastes power and introduces damaging harmonic noise to the wind turbine. The HPS described in this …
An Analysis Of The Relationship Between Economic Development And Demographic Characteristics In The United States, Chad M. Heyne
An Analysis Of The Relationship Between Economic Development And Demographic Characteristics In The United States, Chad M. Heyne
HIM 1990-2015
Over the past several decades there has been extensive research done in an attempt to determine what demographic characteristics affect economic growth, measured in GDP per capita. Understanding what influences the growth of a country will vastly help policy makers enact policies to lead the country in a positive direction. This research focuses on isolating a new variable, women in the work force. As well as isolating a new variable, this research will modify a preexisting variable that was shown to be significant in order to make the variable more robust and sensitive to recessions. The intent of this thesis …
High Yield Assembly And Electron Transport Investigation Of Semiconducting-Rich Local-Gated Carbon Nanotube Field Effect Transistors, Kristy Kormondy
High Yield Assembly And Electron Transport Investigation Of Semiconducting-Rich Local-Gated Carbon Nanotube Field Effect Transistors, Kristy Kormondy
HIM 1990-2015
Single-walled carbon nanotubes (SWNTs) are ideal for use in nanoelectronic devices because of their high current density, mobility and subthreshold swing. However, assembly methods must be developed to reproducibly align all-semiconducting SWNTs at specific locations with individually addressable gates for future integrated circuits. We show high yield assembly of local-gated semiconducting SWNTs assembled via AC-dielectrophoresis (DEP). Using individual local gates and scaling the gate oxide shows faster switching behavior and lower power consumption. The devices were assembled by DEP between prefabricated Pd source and drain electrodes with a thin Al/Al2O3 gate in the middle, and the electrical characteristics were measured …
Size-Effect Of Pd Nanoparticles Supported On Zro2 In The Catalytic Reduction Of No By H2, Young Woo Joh
Size-Effect Of Pd Nanoparticles Supported On Zro2 In The Catalytic Reduction Of No By H2, Young Woo Joh
HIM 1990-2015
Size-selected Pd nanoparticles were synthesized by the reverse-micelle encapsulation method and deposited on a ZrO2 support for the catalytic NO reduction by H2. All of our samples were found to be highly selective, but a significant size effect was not seen for Pd nanoparticles of between 1.2 nm and 5.5 nm. Ultra-small Pd clusters of less than 1 nm were found to be much less active, and are assumed to be affected by an encapsulation effect of the support. Catalyst activity was comparable to that of literature, and is applicable to H2-SCR research.
Estimation For The Cox Model With Various Types Of Censored Data, Tonya Riddlesworth
Estimation For The Cox Model With Various Types Of Censored Data, Tonya Riddlesworth
Electronic Theses and Dissertations
In survival analysis, the Cox model is one of the most widely used tools. However, up to now there has not been any published work on the Cox model with complicated types of censored data, such as doubly censored data, partly-interval censored data, etc., while these types of censored data have been encountered in important medical studies, such as cancer, heart disease, diabetes, etc. In this dissertation, we first derive the bivariate nonparametric maximum likelihood estimator (BNPMLE) F[subscript n](t,z) for joint distribution function F[sub 0](t,z) of survival time T and covariate Z, where T is subject to right censoring, noting …
Modeling Human Group Behavior In Virtual Worlds, Fahad Shah
Modeling Human Group Behavior In Virtual Worlds, Fahad Shah
Electronic Theses and Dissertations
Virtual worlds and massively-multiplayer online games are rich sources of information about large-scale teams and groups, offering the tantalizing possibility of harvesting data about group formation, social networks, and network evolution. They provide new outlets for human social interaction that differ from both face-to-face interactions and non-physically-embodied social networking tools such as Facebook and Twitter. We aim to study group dynamics in these virtual worlds by collecting and analyzing public conversational patterns of users grouped in close physical proximity. To do this, we created a set of tools for monitoring, partitioning, and analyzing unstructured conversations between changing groups of participants …
Effective Task Transfer Through Indirect Encoding, Phillip Verbancsics
Effective Task Transfer Through Indirect Encoding, Phillip Verbancsics
Electronic Theses and Dissertations
An important goal for machine learning is to transfer knowledge between tasks. For example, learning to play RoboCup Keepaway should contribute to learning the full game of RoboCup soccer. Often approaches to task transfer focus on transforming the original representation to fit the new task. Such representational transformations are necessary because the target task often requires new state information that was not included in the original representation. In RoboCup Keepaway, changing from the 3 vs. 2 variant of the task to 4 vs. 3 adds state information for each of the new players. In contrast, this dissertation explores the idea …
Hückel Energy Of A Graph: Its Evolution From Quantum Chemistry To Mathematics, Steven Zimmerman
Hückel Energy Of A Graph: Its Evolution From Quantum Chemistry To Mathematics, Steven Zimmerman
Electronic Theses and Dissertations
The energy of a graph began with German physicist, Erich H¨uckel’s 1931 paper, Quantenttheoretische Beitr¨age zum Benzolproblem. His work developed a method for computing the binding energy of the π-electrons for a certain class of organic molecules. The vertices of the graph represented the carbon atoms while the single edge between each pair of distinct vertices represented the hydrogen bonds between the carbon atoms. In turn, the chemical graphs were represented by an n × n matrix used in solving Schr¨odinger’s eigenvalue/eigenvector equation. The sum of the absolute values of these graph eigenvalues represented the total π-electron energy. The criteria …
Techniques For Boosting The Performance In Content-Based Image Retrieval Systems, Ning Yu
Techniques For Boosting The Performance In Content-Based Image Retrieval Systems, Ning Yu
Electronic Theses and Dissertations
Content-Based Image Retrieval has been an active research area for decades. In a CBIR system, one or more images are used as query to search for similar images. The similarity is measured on the low level features, such as color, shape, edge, texture. First, each image is processed and visual features are extract. Therefore each image becomes a point in the feature space. Then, if two images are close to each other in the feature space, they are considered similar. That is, the k nearest neighbors are considered the most similar images to the query image. In this K-Nearest Neighbor …
Harmony Oriented Architecture, Kyle A. Martin
Harmony Oriented Architecture, Kyle A. Martin
Electronic Theses and Dissertations
This thesis presents Harmony Oriented Architecture: a novel architectural paradigm that applies the principles of Harmony Oriented Programming to the architecture of scalable and evolvable distributed systems. It is motivated by research on Ultra Large Scale systems that has revealed inherent limitations in human ability to design large-scale software systems that can only be overcome through radical alternatives to traditional object-oriented software engineering practice that simplifies the construction of highly scalable and evolvable system. HOP eschews encapsulation and information hiding, the core principles of objectoriented design, in favor of exposure and information sharing through a spatial abstraction. This helps to …
Prediction Of Survival Of Early Stages Lung Cancer Patients Based On Er Beta Cellular Expressions And Epidemiological Data, Evgeny Martinenko
Prediction Of Survival Of Early Stages Lung Cancer Patients Based On Er Beta Cellular Expressions And Epidemiological Data, Evgeny Martinenko
Electronic Theses and Dissertations
We attempted a mathematical model for expected prognosis of lung cancer patients based on a multivariate analysis of the values of ER-interacting proteins (ERbeta) and a membrane bound, glycosylated phosphoprotein MUC1), and patients clinical data recorded at the time of initial surgery. We demonstrate that, even with the limited sample size available to use, combination of clinical and biochemical data (in particular, associated with ERbeta and MUC1) allows to predict survival of lung cancer patients with about 80% accuracy while prediction on the basis of clinical data only gives about 70% accuracy. The present work can be viewed as a …
The Implications Of Virtual Environments In Digital Forensic Investigations, Farrah M. Patterson
The Implications Of Virtual Environments In Digital Forensic Investigations, Farrah M. Patterson
Electronic Theses and Dissertations
This research paper discusses the role of virtual environments in digital forensic investigations. With virtual environments becoming more prevalent as an analysis tool in digital forensic investigations, it’s becoming more important for digital forensic investigators to understand the limitation and strengths of virtual machines. The study aims to expose limitations within commercial closed source virtual machines and open source virtual machines. The study provides a brief overview of history digital forensic investigations and virtual environments, and concludes with an experiment with four common open and closed source virtual machines; the effects of the virtual machines on the host machine as …
Characterization Of Composite Broad Band Absorbing Conjugated Polymer Nanoparticles Using Steady-State, Time-Resolve And Single Particle Spectroscopy, Maxwell Scotland Bonner
Characterization Of Composite Broad Band Absorbing Conjugated Polymer Nanoparticles Using Steady-State, Time-Resolve And Single Particle Spectroscopy, Maxwell Scotland Bonner
Electronic Theses and Dissertations
As the global economy searches for reliable, inexpensive and environmentally friendly renewable energy resources, energy conservation by means of photovoltaics has seen near exponential growth in the last decade. Compared to state-of-the-art inorganic solar cells, organic photovoltaics (OPVs) composed of conjugated polymers are particularly interesting because of their processability, flexibility and the potential for large area devices at a reduced fabrication cost. It has been extensively documented that the interchain and intrachain interactions of conjugated polymers complicate the fundamental understanding of the optical and electronic properties in the solid-state (i.e. thin film active layer). These interactions are highly dependent on …
Bayesian Model Selection For Classification With Possibly Large Number Of Groups, Justin Kyle Davis
Bayesian Model Selection For Classification With Possibly Large Number Of Groups, Justin Kyle Davis
Electronic Theses and Dissertations
The purpose of the present dissertation is to study model selection techniques which are specifically designed for classification of high-dimensional data with a large number of classes. To the best of our knowledge, this problem has never been studied in depth previously. We assume that the number of components p is much larger than the number of samples n, and that only few of those p components are useful for subsequent classification. In what follows, we introduce two Bayesian models which use two different approaches to the problem: one which discards components which have “almost constant” values (Model 1) and …
Ultra High Density Spectral Beam Combining By Thermal Tuning Of Volume Bragg Gratings In Photo-Thermo-Refractive Glass, Derrek Drachenberg
Ultra High Density Spectral Beam Combining By Thermal Tuning Of Volume Bragg Gratings In Photo-Thermo-Refractive Glass, Derrek Drachenberg
Electronic Theses and Dissertations
High power lasers with diffraction limited beam quality are desired for many applications in defense and manufacturing. A lot of applications require laser beams at the 100 kW power level along with divergence close to the diffraction limit. The figure of merit for a beam used in such applications should be radiance which determines the laser power delivered to a remote target. One of the primary limiting factors is thermal distortion of a laser beam caused by excessive heat generated in the laser media. Combination of multiple laser beams is usually considered as a method to mitigate these limitations. Spectral …
Theoretical Study Of Beam Transformations By Volume Diffraction, Sergiy V. Mokhov
Theoretical Study Of Beam Transformations By Volume Diffraction, Sergiy V. Mokhov
Electronic Theses and Dissertations
Laser beams can be manipulated by volume diffractive elements in addition to conventional optical elements like mirrors, lenses, and beam splitters. Conventional optical elements can be described by applying the basic laws of reflection and refraction at the surfaces of the elements. Even diffraction by surface gratings utilizes relatively simple mathematics. This is to be contrasted with the volume diffraction, which requires coupled wave theory in the slowly varying envelope approximation (SVEA) to obtain accurate results. Efficient spatially distributed diffraction of laser beams is possible due to the high coherence of laser light, and it occurs at specific resonant Bragg …
Density Functional Theory Study Of Molecules And Crystals Containing D And F Metals, Shruba Gangopadhyay
Density Functional Theory Study Of Molecules And Crystals Containing D And F Metals, Shruba Gangopadhyay
Electronic Theses and Dissertations
Density Functional Theory (DFT) method is applied to study the crystal structure of transition metal and lanthanide oxides, as well as molecular magnetic complexes. DFT is a widely popular computational approach because it recasts a many-body problem of interacting electrons into an equivalent problem of non-interacting electrons, greatly reducing computational cost. We show that for certain structural properties like phase stability, lattice parameter and oxygen migration energetics pure DFT can give good agreement with experiments. But moving to more sensitive properties like spin state energetic certain modifications of standard DFT are needed. First we investigated mixed ionic-electronic conducting perovskite type …
High Pressure And Micro-Spectroscopic Studies Of Single Living Erythrocytes And The Intraerythrocytic Multplication Cycle Of Plasmodium Falciparum, Silki Arora
Electronic Theses and Dissertations
A novel experimental approach for micro-absorption spectroscopy and high-pressure microscopy of single cells is developed and applied to the investigation of morphological, volume, and spectroscopic changes in healthy red blood cells (RBCs) and erythrocytes infected with the malaria parasite Plasmodium falciparum. Through real-time optical imaging of individual erythrocytes (size ~ 7[micrometer]) we determine the change in volume over the pressure range from 0.1 to 210 MPa. The lateral diameter of healthy RBCs decreases reversibly with pressure with an approximate slope of 0.015 [micrometer] / MPa. In infected cells, clear differences in the deformability and between the compression and decompression curves …
Self-Assembly And Photophysics Of Selected Organic Materials And Two-Photon Bioimaging With Profluorescent Nitroxides, Polyelectrolyte Nanoparticles, And Squaraine Probes, Hyo Yang Ahn
Electronic Theses and Dissertations
Two-photon absorption and upconverted fluorescence has been utilized in a variety of applications in pure science and engineering. Multiphoton-based techniques were used in this research in order to understand photophysical and chemical characteristics of several fluorescent dyes and to demonstrate some of their key applications. Two-photon fluorescence microscopy (2PFM) has become a powerful technique in bio-photonics for non-invasive imaging in the near-infrared (NIR) region (700~1000 nm) that often results in less photobleaching. In Chapter 1, there is a brief introduction to fluorescence, examples of fluorescence materials, and a discussion of the advantages of two-photon absorption. 2PFM imaging was utilized in …
Characterization Of The Nonlinear Refractive Index Of Carbon Disulfide Over An Extended Spectral And Temporal Range, Marcus Seidel
Characterization Of The Nonlinear Refractive Index Of Carbon Disulfide Over An Extended Spectral And Temporal Range, Marcus Seidel
Electronic Theses and Dissertations
The intensity dependent refractive index change of a medium is frequently described in terms of the product n₂ · I where n₂ is the nonlinear refractive index and I the light intensity. The nonlinear refractive index is often treated as constant which is a reasonable assumption if the light interacts only with bound electrons. In the case of carbon disulfide (CS₂) however, nuclear motions contribute to n₂. These motions occur on the sub picosecond time scale and thus become especially relevant for ultrashort laser pulses. The neat liquid CS₂ is studied because it exhibits a large nonlinear refractive index in …
An Approach To Improve The Failure Rate Model Of A Solid State Laser By Utalizing The Physics Of Failure Methodology, Omar L. Thompson
An Approach To Improve The Failure Rate Model Of A Solid State Laser By Utalizing The Physics Of Failure Methodology, Omar L. Thompson
Electronic Theses and Dissertations
The ability to predict the failure rate of any military laser is very critical. In-field laser usage does not support the troubleshooting and repairing of a complex electro optical system. The only published laser failure rate model was last updated by the Department of Defense in 1975. Consequently, the failure rate predicted is inaccurate due to model deficiencies. This dissertation has developed a laser failure rate model for diode pumped lasers with improved failure rate prediction accuracy. The model has surpassed the capabilities of the Department of Defense model by the inclusion of key performance attributes that are currently not …
Innovative Pollutant Load Monitoring, Eric Gurr
Innovative Pollutant Load Monitoring, Eric Gurr
Electronic Theses and Dissertations
Modern streamflow measuring equipment, water quality sampling techniques and a better understanding of pollutant washoff are continuously being developed as today's society is in critical need of improving water management, minimizing developmental impacts and preventing environmental hazards. In particular, the study of the spatial, temporal and volumetric characteristics of annual pollutant loading caused by variations in precipitation, land use and other anthropogenic factors is of great significance due to their relation to future global water demands. The research presented here falls in three parts. In the first part of the dissertation, an acoustical Doppler velocity profiler installed in a submerged …
Computational Study Of The Near Field Spontaneous Creation Of Photonic States Coupled To Few Level Systems, Sergio Tafur
Computational Study Of The Near Field Spontaneous Creation Of Photonic States Coupled To Few Level Systems, Sergio Tafur
Electronic Theses and Dissertations
Models of the spontaneous emission and absorption of photons coupled to the electronic states of quantum dots, molecules, N-V (single nitrogen vacancy) centers in diamond, that can be modeled as artificial few level atoms, are important to the development of quantum computers and quantum networks. A quantum source modeled after an effective few level system is strongly dependent on the type and coupling strength the allowed transitions. These selection rules are subject to the Wigner-Eckert theorem which specifies the possible transitions during the spontaneous creation of a photonic state and its subsequent emission. The model presented in this dissertation describes …
Infrared Emission Spectroscopy Of Hot Carbon Monoxide, Farnood Khalilzadeh Rezaie
Infrared Emission Spectroscopy Of Hot Carbon Monoxide, Farnood Khalilzadeh Rezaie
Electronic Theses and Dissertations
Gas giant exoplanets known as hot Jupiters orbit close to their parent stars and are heated to high temperatures. Their infrared spectra, measured by photometry during secondary eclipses, are dominated by carbon monoxide and methane, the principle reservoirs of carbon on these planets. The relative CO and CH4 abundances inform us about temperature and pressure conditions and also about mixing by global winds driven by intense but asymmetric heating for these tidally locked bodies. Emission spectra collected during secondary eclipses, as the hot Jupiter passes behind its parent star, in principle allows a determination of the CO:CH4 concentration ratio. Since …
Perceptual Image Quality Of Launch Vehicle Imaging Telescopes, Joshua K. Lentz
Perceptual Image Quality Of Launch Vehicle Imaging Telescopes, Joshua K. Lentz
Electronic Theses and Dissertations
A large fleet (in the hundreds) of high quality telescopes are used for tracking and imaging of launch vehicles during ascent from Cape Canaveral Air Force Station and Kennedy Space Center. A maintenance tool has been development for use with these telescopes. The tool requires rankings of telescope condition in terms of the ability to generate useful imagery. It is thus a case of ranking telescope conditions on the basis of the perceptual image quality of their imagery. Perceptual image quality metrics that are well-correlated to observer opinions of image quality have been available for several decades. However, these are …
Price Discovery In The U.S. Bond Market Trading Strategies And The Cost Of Liquidity, Haimei Shao
Price Discovery In The U.S. Bond Market Trading Strategies And The Cost Of Liquidity, Haimei Shao
Electronic Theses and Dissertations
The world bond market is nearly twice as large as the equity market. The goal of this dissertation is to study the dynamics of bond price. Among the liquidity risk, interest rate risk and default risk, this dissertation will focus on the liquidity risk and trading strategy. Under the mathematical frame of stochastic control, we model price setting in U.S. bond markets where dealers have multiple instruments to smooth inventory imbalances. The difficulty in obtaining the optimal trading strategy is that the optimal strategy and value function depend on each other, and the corresponding HJB equation is nonlinear. To solve …
Fractal Spectral Measures In Two Dimensions, Beng Oscar Alrud
Fractal Spectral Measures In Two Dimensions, Beng Oscar Alrud
Electronic Theses and Dissertations
We study spectral properties for invariant measures associated to affine iterated function systems. We present various conditions under which the existence of a Hadamard pair implies the existence of a spectrum for the fractal measure. This solves a conjecture proposed by Dorin Dutkay and Palle Jorgensen, in several special cases in dimension 2.
Single-Electron Transport Spectroscopy Studies Of Magnetic Molecules And Nanoparticles, Firoze Haque
Single-Electron Transport Spectroscopy Studies Of Magnetic Molecules And Nanoparticles, Firoze Haque
Electronic Theses and Dissertations
Magnetic nanoparticles and molecules, in particular ferromagnetic noble metal nanoparticles, molecular magnet and single-molecule magnets (SMM), are perfect examples to investigate the role of quantum mechanics at the nanoscale. For example, SMMs are known to reverse their magnetization by quantum tunneling in the absence of thermal excitation and show a number of fundamental quantum mechanical manifestations, such as quantum interference effects. On the other hand, noble metal nanoparticles are found to behave ferromagnetically for diameters below a few nanometers. Some of these manifestations are still intriguing, and novel research approaches are necessary to advance towards a more complete understanding of …