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A Review On N-Doped Biochar For Oxidative Degradation Of Organic Contaminants In Wastewater By Persulfate Activation, Yaxuan Gao, Wenran Gao, Haonan Zhu, Haoran Chen, Shanshan Yan, Ming Zhao, Hongqi Sun, Junjie Zhang, Shu Zhang
A Review On N-Doped Biochar For Oxidative Degradation Of Organic Contaminants In Wastewater By Persulfate Activation, Yaxuan Gao, Wenran Gao, Haonan Zhu, Haoran Chen, Shanshan Yan, Ming Zhao, Hongqi Sun, Junjie Zhang, Shu Zhang
Research outputs 2022 to 2026
The Persulfate-based advanced oxidation process is the most efficient and commonly used technology to remove organic contaminants in wastewater. Due to the large surface area, unique electronic properties, abundant N functional groups, cost-effectiveness, and environmental friendliness, N-doped biochars (NBCs) are widely used as catalysts for persulfate activation. This review focuses on the NBC for oxidative degradation of organics-contaminated wastewater. Firstly, the preparation and modification methods of NBCs were reviewed. Then the catalytic performance of NBCs and modified NBCs on the oxidation degradation of organic contaminants were discussed with an emphasis on the degradation mechanism. We further summarized the detection technologies …
Wastewater Remediation Technologies Using Macroscopic Graphene-Based Materials: A Perspective, Rajan Arjan Kalyan Hirani, Abdul Hannan Asif, Nasir Rafique, Lei Shi, Shu Zhang, Hong Wu, Hongqi Sun
Wastewater Remediation Technologies Using Macroscopic Graphene-Based Materials: A Perspective, Rajan Arjan Kalyan Hirani, Abdul Hannan Asif, Nasir Rafique, Lei Shi, Shu Zhang, Hong Wu, Hongqi Sun
Research outputs 2014 to 2021
Three-dimensional (3D) graphene-based macrostructures are being developed to combat the issues associated with two-dimensional (2D) graphene materials in practical applications. The 3D macrostructures (3DMs), for example, membranes, fibres, sponges, beads, and mats, can be formed by the self-assembly of 2D graphene-based precursors with exceptional surface area and unique chemistry. With rational design, the 3D macrostructures can then possess outstanding properties and exclusive structures. Thanks to various advantages, these macrostructures are competing in a variety of applications with promising performances unlike the traditional activated carbons, biochars and hydrochars, which have less flexibilities for modifications towards versatile applications. However, despite having such …
Preparation Of Activated Biochar-Supported Magnetite Composite For Adsorption Of Polychlorinated Phenols From Aqueous Solutions, Byung-Moon Jun, Yejin Kim, Jonghun Han, Yeomin Yoon, Chang Min Park
Preparation Of Activated Biochar-Supported Magnetite Composite For Adsorption Of Polychlorinated Phenols From Aqueous Solutions, Byung-Moon Jun, Yejin Kim, Jonghun Han, Yeomin Yoon, Chang Min Park
Faculty Publications
For this study, we applied activated biochar (AB) and its composition with magnetite (AB-Fe3O4) as adsorbents for the removal of polychlorophenols in model wastewater. We comprehensively characterized these adsorbents and performed adsorption tests under several experimental parameters. Using FTIR, we confirmed successful synthesis of AB-Fe3O4 composite through cetrimonium bromide surfactant. We conducted adsorption tests using AB and AB-Fe3O4 to treat model wastewater containing polychlorophenols, such as 2,3,4,6-Tetrachlorophenol (TeCP), 2,4,6-Trichlorophenol (TCP), and 2,4-Dichlorophenol (DCP). Results of the isotherm and the kinetic experiments were well adapted to Freundlich’s isotherm model and the …
Spatially Explicit Life Cycle Assessment: Opportunities And Challenges Of Wastewater-Based Algal Biofuels In The United States, Javad Roostaei, Yongli Zhang
Spatially Explicit Life Cycle Assessment: Opportunities And Challenges Of Wastewater-Based Algal Biofuels In The United States, Javad Roostaei, Yongli Zhang
Civil and Environmental Engineering Faculty Research Publications
This work presented a Spatially-Explicit-High-Resolution Life Cycle Assessment (SEHR-LCA) model for wastewater-based algal biofuel production, by integrating life cycle assessment, GIS analysis, and site-specific Wastewater Treatment Plants (WWTPs) data analysis. Wastewater resources, land availability, and meteorological variation were analyzed for algae cultivation. Three pathways, Microwave Pyrolysis, hydrothermal liquefaction, and lipid extraction were modeled for bio-oil conversion. This model enables the assessment of seasonal and site-specific variations in productivity and environmental impacts of wastewater-based algal bio-oil across the whole U.S. Model results indicate that wastewater-based algal bio-oil can provide an opportunity to increase national biofuel output. The potential production of algal …
Emerging Investigators Series: Pyrolysis Removes Common Microconstituents Triclocarban, Triclosan, And Nonylphenol From Biosolids, J. J. Ross, Daniel Zitomer, T. R. Miller, C. A. Weirich, Patrick J. Mcnamara
Emerging Investigators Series: Pyrolysis Removes Common Microconstituents Triclocarban, Triclosan, And Nonylphenol From Biosolids, J. J. Ross, Daniel Zitomer, T. R. Miller, C. A. Weirich, Patrick J. Mcnamara
Civil and Environmental Engineering Faculty Research and Publications
Reusing biosolids is vital for the sustainability of wastewater management. Pyrolysis is an anoxic thermal degradation process that can be used to convert biosolids into energy rich py-gas and py-oil, and a beneficial soil amendment, biochar. Batch biosolids pyrolysis (60 minutes) revealed that triclocarban and triclosan were removed (to below quantification limit) at 200 °C and 300 °C, respectively. Substantial removal (>90%) of nonylphenol was achieved at 300 °C as well, but 600 °C was required to remove nonylphenol to below the quantification limit. At 500 °C, the pyrolysis reaction time to remove >90% of microconstituents was less than …