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Synthesis, Structure, And Catalytic Properties Of Size-Selected Platinum Nanoparticles, Simon Armando Covone
Synthesis, Structure, And Catalytic Properties Of Size-Selected Platinum Nanoparticles, Simon Armando Covone
Electronic Theses and Dissertations
The use of heterogeneous catalysis is well established in chemical synthesis, energy, and environmental engineering applications. Supported Pt nanoparticles have been widely reported to act as catalysts in a vast number of chemical reactions. In this report, the performance of Pt/ZrO2 nanocatalyst for the decomposition of methanol, ethanol, 2-propanol, and 2-butanol is investigated. The potential of each alcohol for the production of H2 and other relevant products in the presence of a catalyst is studied. All the alcohols studied show some decomposition activity below 200°C which increased with increasing temperature. In all cases, high selectivity towards H2 formation is observed. …
Plasmon Enhanced Near-Field Interactions In Surface Coupled Nanoparticle Arrays For Integrated Nanophotonic Devices, Amitabh Ghoshal
Plasmon Enhanced Near-Field Interactions In Surface Coupled Nanoparticle Arrays For Integrated Nanophotonic Devices, Amitabh Ghoshal
Electronic Theses and Dissertations
The current thrust towards developing silicon compatible integrated nanophotonic devices is driven by need to overcome critical challenges in electronic circuit technology related to information bandwidth and thermal management. Surface plasmon nanophotonics represents a hybrid technology at the interface of optics and electronics that could address several of the existing challenges. Surface plasmons are electronic charge density waves that can occur at a metal-dielectric interface at optical and infrared frequencies. Numerous plasmon based integrated optical devices such as waveguides, splitters, resonators and multimode interference devices have been developed, however no standard integrated device for coupling light into nanoscale optical circuits …